Hydrogen production from liquid hydrocarbon fuels for PEMFC application
文献类型：期刊论文
| 作者 | Chen, Yazhong; Xu, Hengyong; Wang, Yuzhong; Jin, Xianglan; Xiong, Guoxing |
| 刊名 | fuel processing technology
 |
| 出版日期 | 2006-11-01 |
| 卷号 | 87期号:11页码:971-978 |
| 关键词 | liquid hydrocarbons prereforming autothermal reforming distributed air feed nickel catalyst Pd membrane |
| 产权排序 | 1;1 |
| 通讯作者 | 熊国兴 |
| 英文摘要 | lack of efficient hydrogen storage intermediate has boosted the development of fuel processor or economic onsite hydrogen production techniques for application to proton exchange membrane fuel cell promptly. aiming to develop onsite hydrogen production techniques for proton exchange membrane fuel cell application using nickel-based reforming catalysts and stainless steel reactors, in this paper, a novel process for h-2 production from liquid hydrocarbon fuels was proposed and experimentally demonstrated on a lab scale. the main operations involved prereforming, autothermal reforming, high temperature water gas shift, low temperature water gas shift and h-2 enrichment by pd membrane. the results indicated that prereforming introduction prior to autothermal reforming suppressed undesired gas phase reactions efficiently and made reforming reactions perform catalytically and smoothly, which was confirmed by a stable 500 h time-on-stream test of both prereforming and autothermal reforming catalysts. the air distributed feed applied in autothermal reforming reactor coupled the endothermic steam reforming and exothermic catalytic combustion reactions over the catalyst closely, maintaining an appropriate temperature distribution curve for autothermal reforming catalyst bed. during the process of h-2 enrichment by highly h-2 permeable pd composite membrane, concentration polarization played an important role. (c) 2006 elsevier b.v. all rights reserved. |
| WOS标题词 | science & technology ; physical sciences ; technology |
| 类目[WOS] | chemistry, applied ; energy & fuels ; engineering, chemical |
| 研究领域[WOS] | chemistry ; energy & fuels ; engineering |
| 关键词[WOS] | gas-production ; cell systems ; separation ; catalysts |
| 收录类别 | SCI |
| 原文出处 | true |
| 语种 | 英语 |
| WOS记录号 | WOS:000241960300004 |
| 公开日期 | 2010-11-30 |
| 源URL | [http://159.226.238.44/handle/321008/97651]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Appl Catalysis Lab, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 3.Res Inst Daqing Petrohem Co, Daqing 163000, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Yazhong,Xu, Hengyong,Wang, Yuzhong,et al. Hydrogen production from liquid hydrocarbon fuels for PEMFC application[J]. fuel processing technology,2006,87(11):971-978. |
| APA | Chen, Yazhong,Xu, Hengyong,Wang, Yuzhong,Jin, Xianglan,&Xiong, Guoxing.(2006).Hydrogen production from liquid hydrocarbon fuels for PEMFC application.fuel processing technology,87(11),971-978. |
| MLA | Chen, Yazhong,et al."Hydrogen production from liquid hydrocarbon fuels for PEMFC application".fuel processing technology 87.11(2006):971-978. |
入库方式： OAI收割
来源：大连化学物理研究所
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