Highly dispersed molybdenum oxide supported on HZSM-5 for methane dehydroaromatization
文献类型：期刊论文
| 作者 | Sun, Changyong1,2; Yao, Songdong1; Shen, Wenjie1; Lin, Liwu1 |
| 刊名 | catalysis letters
 |
| 出版日期 | 2008-04-01 |
| 卷号 | 122期号:1-2页码:84-90 |
| 关键词 | Mo/HZSM-5 ammonia solution methane dehydroaromatization stability |
| 产权排序 | 1;1 |
| 通讯作者 | 申文杰 ; 林励吾 |
| 英文摘要 | mo/hzsm-5 catalyst with highly dispersed moo (x) species was prepared by adding ammonia solution to the ammonium heptamolybdate aqueous solution during the impregnation process. compared with the large mo7o246- species which is predominantly presented in the conventional impregnation solution, the monomer moo42- formed in ammonia solution could efficiently diffuse into the micropores and/or channels of the hzsm-5, resulting in higher dispersion of mo species as well as enhanced interaction with the surface -oh groups of hzsm-5. consequently, the obtained mo/hszm-5 catalyst showed rather high catalytic stability and greatly enhanced selectivity towards benzene for methane dehydroaromatization reaction by effectively inhibiting the coke formation. |
| WOS标题词 | science & technology ; physical sciences |
| 类目[WOS] | chemistry, physical |
| 研究领域[WOS] | chemistry |
| 关键词[WOS] | hydrothermal post-synthesis ; nonoxidative conditions ; mo/hzsm-5 catalysts ; coke-resistance ; aromatization ; zeolite ; conversion ; silanation ; mo/h-zsm5 ; enhance |
| 收录类别 | SCI |
| 原文出处 | true |
| 语种 | 英语 |
| WOS记录号 | WOS:000253754800013 |
| 公开日期 | 2010-11-30 |
| 源URL | [http://159.226.238.44/handle/321008/99951]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 2.Shantou Univ, Dept Chem, Shantou 515063, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Changyong,Yao, Songdong,Shen, Wenjie,et al. Highly dispersed molybdenum oxide supported on HZSM-5 for methane dehydroaromatization[J]. catalysis letters,2008,122(1-2):84-90. |
| APA | Sun, Changyong,Yao, Songdong,Shen, Wenjie,&Lin, Liwu.(2008).Highly dispersed molybdenum oxide supported on HZSM-5 for methane dehydroaromatization.catalysis letters,122(1-2),84-90. |
| MLA | Sun, Changyong,et al."Highly dispersed molybdenum oxide supported on HZSM-5 for methane dehydroaromatization".catalysis letters 122.1-2(2008):84-90. |
入库方式： OAI收割
来源：大连化学物理研究所
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