Highlights of major progress on single-atom catalysis in 2017
文献类型：期刊论文
| 作者 | Guo, Yalin1,2; Lang, Rui1; Qiao, Botao1 |
| 刊名 | Catalysts
 |
| 出版日期 | 2019-02-01 |
| 卷号 | 9期号:2页码:12 |
| 关键词 | Single-atom catalysis Catalyst fabrication C1 chemical conversion Strong metal-support interaction Reaction mechanism |
| ISSN号 | 2073-4344 |
| DOI | 10.3390/catal9020135 |
| 通讯作者 | Qiao, botao(bqiao@dicp.ac.cn) |
| 英文摘要 | Single-atom catalysis has rapidly progressed during the last few years. in 2017, single-atom catalysts (sacs) were fabricated with higher metal loadings and designed into more delicate structures. sacs also found wide applications in c1 chemical conversion, such as selective oxidation of methane and conversion of carbon dioxide. both experimental characterizations and computational modeling revealed the presence of tunable interactions between single atom species and their surrounding chemical environment, and thus sacs may be more effective and more stable than their nanoparticle counterparts. in this mini-review, we summarize the major achievements of sacs into three main aspects: (a) the advanced synthetic methodologies, (b) catalytic performance in c1 chemistry, and (c) strong metal-support interaction induced unexpected durability. these accomplishments will shed new light on the recognition of single-atom catalysis and encourage more efforts to explore potential applications of sacs. |
| WOS关键词 | OXYGEN REDUCTION REACTION ; METAL-ORGANIC FRAMEWORKS ; FE-N-C ; SELECTIVE HYDROGENATION ; PHOTOCATALYTIC DEGRADATION ; EFFICIENT ELECTROCATALYST ; PLATINUM CATALYSTS ; ACTIVE-SITES ; OXIDATION ; CARBON |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Physical |
| 语种 | 英语 |
| WOS记录号 | WOS:000460702200029 |
| 出版者 | MDPI |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2372681 |
| 专题 | 大连化学物理研究所 |
| 通讯作者 | Qiao, Botao |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Guo, Yalin,Lang, Rui,Qiao, Botao. Highlights of major progress on single-atom catalysis in 2017[J]. Catalysts,2019,9(2):12. |
| APA | Guo, Yalin,Lang, Rui,&Qiao, Botao.(2019).Highlights of major progress on single-atom catalysis in 2017.Catalysts,9(2),12. |
| MLA | Guo, Yalin,et al."Highlights of major progress on single-atom catalysis in 2017".Catalysts 9.2(2019):12. |
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来源：大连化学物理研究所
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