中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Two-dimensional (pea)(2)pbbr4 perovskite single crystals for a high performance uv-detector

文献类型:期刊论文

作者Zhang, Yunxia1; Liu, Yucheng1; Xu, Zhuo1; Ye, Haochen1; Li, Qingxian1; Hu, Mingxin1; Yang, Zhou1; Liu, Shengzhong (Frank)1,2
刊名Journal of materials chemistry c
出版日期2019-02-14
卷号7期号:6页码:1584-1591
ISSN号2050-7526
DOI10.1039/c8tc06129g
通讯作者Yang, zhou(zyang@snnu.edu.cn) ; Liu, shengzhong (frank)(szliu@dicp.ac.cn)
英文摘要Two-dimensional (2d) metal halide perovskites have shown great potential in high performance optoelectronic applications due to their intrinsic quantum well structure, enhanced moisture- and photo-stability. unfortunately, there is still no effective method to produce large-size 2d hybrid perovskite single crystals, and consequently there is lack of research on its optoelectronic applications. herein, we report the utilization of a controlled evaporation process to grow well-defined large-size (>200 mm(2)) 2d (pea)(2)pbbr4 (c6h5ch2ch2nh3+, pea(+)) single crystals. upon careful examination of the crystal growth kinetics, it was found that the optimum temperature for the growth of (pea)(2)pbbr4 single crystal wafer was 23 +/- 0.5 degrees c. the wafers that were harvested showed high mu-tau () product, superior environmental stability and irradiation resistance. furthermore, an array of planar-type uv photodetectors were designed and fabricated with extremely low dark current (approximate to 10(-13) a), large on/off current ratio (approximate to 10(5)), very high specific detectivity (approximate to 10(13) cm hz(1/2) w-1) and fast response rate (approximate to 0.4 ms). all the above performance data are among the best achieved compared to those of the state-of-the-art materials including zno, tio2 and gan in the field. it makes us believe that the availability of these materials may pave the way for ultrafast optical computing and optical communications.
WOS关键词GROWTH
WOS研究方向Materials Science ; Physics
WOS类目Materials Science, Multidisciplinary ; Physics, Applied
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000459572600013
URI标识http://www.irgrid.ac.cn/handle/1471x/2372797
专题大连化学物理研究所
通讯作者Yang, Zhou; Liu, Shengzhong (Frank)
作者单位1.Shaanxi Normal Univ, Shaanxi Engn Lab Adv Energy Technol,Sch Mat Sci &, Key Lab Appl Surface & Colloid Chem,Minist Educ, Shaanxi Key Lab Adv Energy Devices,Inst Adv Energ, Xian 710119, Shaanxi, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, IChEM, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Yunxia,Liu, Yucheng,Xu, Zhuo,et al. Two-dimensional (pea)(2)pbbr4 perovskite single crystals for a high performance uv-detector[J]. Journal of materials chemistry c,2019,7(6):1584-1591.
APA Zhang, Yunxia.,Liu, Yucheng.,Xu, Zhuo.,Ye, Haochen.,Li, Qingxian.,...&Liu, Shengzhong .(2019).Two-dimensional (pea)(2)pbbr4 perovskite single crystals for a high performance uv-detector.Journal of materials chemistry c,7(6),1584-1591.
MLA Zhang, Yunxia,et al."Two-dimensional (pea)(2)pbbr4 perovskite single crystals for a high performance uv-detector".Journal of materials chemistry c 7.6(2019):1584-1591.

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来源:大连化学物理研究所

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