Ir-based bimetallic catalysts for hydrogen production through glycerol aqueous-phase reforming
文献类型：期刊论文
| 作者 | Espinosa-Moreno, Francisco1; Balla, Putrakumar2; Shen, Wenjie2; Chavarria-Hernandez, Juan C.1; Ruiz-Gomez, Miguel3; Tlecuitl-Beristain, Saul4 |
| 刊名 | Catalysts
 |
| 出版日期 | 2018-12-01 |
| 卷号 | 8期号:12页码:16 |
| 关键词 | Iridium Glycerol Aqueous-phase reforming Hydrogen production |
| ISSN号 | 2073-4344 |
| DOI | 10.3390/catal8120613 |
| 通讯作者 | Chavarria-hernandez, juan c.(jc.ch@cicy.mx) |
| 英文摘要 | Iridium, iridium-nickel and iridium-copper catalysts were prepared by incipient wetness impregnation and evaluated in the aqueous-phase reforming of glycerol using la2o3 or ceo2 as supports. the catalysts were characterized by n-2 physisorption, xrd, h-2-tpr, xps, and eds. the reactions were carried out in a fixed bed reactor feeding a solution of glycerol (10 wt %) in water, at 270 degrees c and 58 bar. all irni catalysts showed higher activity than ir and ircu, and in general, la2o3 catalysts showed a better performance when compared to ceo2 catalysts. the highest hydrogen production yield was reached by bimetallic irni catalysts with over 250 mu mol min(-1) g(cat)(-1) for la2o3 and 150 mu mol min(-1) g(cat)(-1) for ceo2. |
| WOS关键词 | ETHYLENE-GLYCOL ; FOSSIL-FUELS ; IR/CEO2 CATALYSTS ; ETHANOL ; NI ; HYDROCARBONS ; DEPLETION ; METHANOL ; RE ; PERFORMANCE |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Physical |
| 语种 | 英语 |
| WOS记录号 | WOS:000454711500045 |
| 出版者 | MDPI |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2372886 |
| 专题 | 大连化学物理研究所 |
| 通讯作者 | Chavarria-Hernandez, Juan C. |
| 作者单位 | 1.Parque Cient & Tecnol Yucatan, Ctr Invest Cient Yucatan, Carretera Sierra Papacal Chuburna Puerto, Merida 97302, Yucatan, Mexico 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhong Shan Rd, Dalian 116023, Peoples R China 3.CONACYT CINVESTAV IPN, CONACYT Dept Fis Aplicada, Merida 97310, Yucatan, Mexico 4.Univ Politecn Tlaxcala, Ingn Biotecnol, Tepeyanco 90180, Tlaxcala, Mexico |
| 推荐引用方式 GB/T 7714 | Espinosa-Moreno, Francisco,Balla, Putrakumar,Shen, Wenjie,et al. Ir-based bimetallic catalysts for hydrogen production through glycerol aqueous-phase reforming[J]. Catalysts,2018,8(12):16. |
| APA | Espinosa-Moreno, Francisco,Balla, Putrakumar,Shen, Wenjie,Chavarria-Hernandez, Juan C.,Ruiz-Gomez, Miguel,&Tlecuitl-Beristain, Saul.(2018).Ir-based bimetallic catalysts for hydrogen production through glycerol aqueous-phase reforming.Catalysts,8(12),16. |
| MLA | Espinosa-Moreno, Francisco,et al."Ir-based bimetallic catalysts for hydrogen production through glycerol aqueous-phase reforming".Catalysts 8.12(2018):16. |
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来源：大连化学物理研究所
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