Visible-light driven overall conversion of co2 and h2o to ch4 and o-2 on 3d-sic@2d-mos2 heterostructure
文献类型：期刊论文
| 作者 | Wang, Ying1,2; Zhang, Zizhong1; Zhang, Lina1; Luo, Zhongbin1; Shen, Jinni1; Lin, Huaxiang1; Long, Jinlin1; Wu, Jeffrey C. S.3; Fu, Xianzhi1; Wang, Xuxu1 |
| 刊名 | Journal of the american chemical society
 |
| 出版日期 | 2018-11-07 |
| 卷号 | 140期号:44页码:14595-14598 |
| ISSN号 | 0002-7863 |
| DOI | 10.1021/jacs.8b09344 |
| 通讯作者 | Zhang, zizhong(z.zhang@fzu.edu.cn) ; Wang, xuxu(xwang@fzu.edu.cn) ; Li, can(canli@dicp.ac.cn) |
| 英文摘要 | A marigold-like sic@mos2 nanoflower with a unique z-scheme structure efficiently achieves the overall conversion of gas phase co2 with h2o (co2 (g) + 2h(2)o (g) = ch4 + 2o(2)) without any sacrificial reagents under visible light (lambda >= 420 nm) irradiation. the ch4 and o-2 evolution are 323 and 621 mu l-g-(1).h(-1), and stable throughout 5 cycle reactions of total 40 h. this work demonstrates a breakthrough in artificial photosynthesis with the z-scheme 1d heterojunction constructed by combining 2d semiconductor and 3d semiconductor based on the transfer balance of photogenerated electron and hole. |
| WOS关键词 | PHOTOCATALYTIC H-2 PRODUCTION ; OXYGEN-ISOTOPE EXCHANGE ; CARRIER MOBILITY ; REDUCTION ; OXIDATION ; PHOTOREDUCTION ; PERFORMANCE ; HYDROGEN ; TIO2 |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Multidisciplinary |
| 语种 | 英语 |
| WOS记录号 | WOS:000449887800015 |
| 出版者 | AMER CHEMICAL SOC |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2373069 |
| 专题 | 大连化学物理研究所 |
| 通讯作者 | Zhang, Zizhong; Wang, Xuxu; Li, Can |
| 作者单位 | 1.Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350108, Fujian, Peoples R China 2.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Inorgan Synthet & Appl Chem, State Key Lab Base Ecochem Engn, Qingdao 266042, Peoples R China 3.Natl Taiwan Univ, Dept Chem Engn, Taipei 10617, Taiwan 4.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Ying,Zhang, Zizhong,Zhang, Lina,et al. Visible-light driven overall conversion of co2 and h2o to ch4 and o-2 on 3d-sic@2d-mos2 heterostructure[J]. Journal of the american chemical society,2018,140(44):14595-14598. |
| APA | Wang, Ying.,Zhang, Zizhong.,Zhang, Lina.,Luo, Zhongbin.,Shen, Jinni.,...&Li, Can.(2018).Visible-light driven overall conversion of co2 and h2o to ch4 and o-2 on 3d-sic@2d-mos2 heterostructure.Journal of the american chemical society,140(44),14595-14598. |
| MLA | Wang, Ying,et al."Visible-light driven overall conversion of co2 and h2o to ch4 and o-2 on 3d-sic@2d-mos2 heterostructure".Journal of the american chemical society 140.44(2018):14595-14598. |
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来源：大连化学物理研究所
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