Using stable isotopes to trace sources and formation processes of sulfate aerosols from beijing, china
文献类型：期刊论文
| 作者 | Han, Xiaokun1,2; Guo, Qingjun1; Liu, Congqiang3; Fu, Pingqing4; Strauss, Harald5; Yang, Junxing1; Hu, Jian3; Wei, Lianfang4; Ren, Hong4; Peters, Marc1 |
| 刊名 | Scientific reports
 |
| 出版日期 | 2016-07-20 |
| 卷号 | 6页码:14 |
| ISSN号 | 2045-2322 |
| DOI | 10.1038/srep29958 |
| 通讯作者 | Guo, qingjun(guoqj@igsnrr.ac.cn) |
| 英文摘要 | Particulate pollution from anthropogenic and natural sources is a severe problem in china. sulfur and oxygen isotopes of aerosol sulfate (delta s-34(sulfate) and delta o-18(sulfate)) and water-soluble ions in aerosols collected from 2012 to 2014 in beijing are being utilized to identify their sources and assess seasonal trends. the mean delta s-34 value of aerosol sulfate is similar to that of coal from north china, indicating that coal combustion is a significant contributor to atmospheric sulfate. the delta s-34(sulfate) and delta(18)o(sulfate)values are positively correlated and display an obvious seasonality (high in winter and low in summer). although an influence of meteorological conditions to this seasonality in isotopic composition cannot be ruled out, the isotopic evidence suggests that the observed seasonality reflects temporal variations in the two main contributions to beijing aerosol sulfate, notably biogenic sulfur emissions in the summer and the increasing coal consumption in winter. our results clearly reveal that a reduction in the use of fossil fuels and the application of desulfurization technology will be important for effectively reducing sulfur emissions to the beijing atmosphere. |
| WOS关键词 | CLOUD CONDENSATION NUCLEI ; GAS-PHASE OXIDATION ; WET PRECIPITATION ; AMMONIUM-SULFATE ; SULFUR ISOTOPES ; ORGANIC-CARBON ; ATMOSPHERE ; FRACTIONATION ; PM2.5 ; JAPAN |
| WOS研究方向 | Science & Technology - Other Topics |
| WOS类目 | Multidisciplinary Sciences |
| 语种 | 英语 |
| 出版者 | NATURE PUBLISHING GROUP |
| WOS记录号 | WOS:000379918100001 |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2374604 |
| 专题 | 中国科学院大学 |
| 通讯作者 | Guo, Qingjun |
| 作者单位 | 1.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Ctr Environm Remediat, Beijing 100101, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Guizhou, Peoples R China 4.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China 5.Univ Munster, Inst Geol & Palaontol, Corrensstr 24, D-48149 Munster, Germany |
| 推荐引用方式 GB/T 7714 | Han, Xiaokun,Guo, Qingjun,Liu, Congqiang,et al. Using stable isotopes to trace sources and formation processes of sulfate aerosols from beijing, china[J]. Scientific reports,2016,6:14. |
| APA | Han, Xiaokun.,Guo, Qingjun.,Liu, Congqiang.,Fu, Pingqing.,Strauss, Harald.,...&Tian, Liyan.(2016).Using stable isotopes to trace sources and formation processes of sulfate aerosols from beijing, china.Scientific reports,6,14. |
| MLA | Han, Xiaokun,et al."Using stable isotopes to trace sources and formation processes of sulfate aerosols from beijing, china".Scientific reports 6(2016):14. |
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来源：中国科学院大学
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