Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid
文献类型:期刊论文
作者 | Wang, Wangyin1; Wang, Hong1,2; Zhu, Qingjun2,3; Qin, Wei1; Han, Guangye3; Shen, Jian-Ren3,4; Zong, Xu1; Li, Can1 |
刊名 | Angewandte chemie-international edition
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出版日期 | 2016-08-01 |
卷号 | 55期号:32页码:9229-9233 |
关键词 | Photocatalysis Photoelectrochemistry Photosystem ii Water splitting Z-scheme |
ISSN号 | 1433-7851 |
DOI | 10.1002/anie.201604091 |
通讯作者 | Zong, xu(xzong@dicp.ac.cn) ; Li, can(canli@dicp.ac.cn) |
英文摘要 | Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. a natural-artificial photosynthetic hybrid platform is formed by wiring photosystem ii (psii) and a platinum-decorated silicon photoelectrochemical (pec) cell in a tandem manner based on a photocatalytic-pec z-scheme design. although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. moreover, h-2 and o-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional z-scheme design. furthermore, the tandem configuration and the spatial separation between psii and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems. |
WOS关键词 | PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION |
WOS研究方向 | Chemistry |
WOS类目 | Chemistry, Multidisciplinary |
语种 | 英语 |
WOS记录号 | WOS:000383371800017 |
出版者 | WILEY-V C H VERLAG GMBH |
URI标识 | http://www.irgrid.ac.cn/handle/1471x/2376206 |
专题 | 中国科学院大学 |
通讯作者 | Zong, Xu; Li, Can |
作者单位 | 1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China 4.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan |
推荐引用方式 GB/T 7714 | Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid[J]. Angewandte chemie-international edition,2016,55(32):9229-9233. |
APA | Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid.Angewandte chemie-international edition,55(32),9229-9233. |
MLA | Wang, Wangyin,et al."Spatially separated photosystem ii and a silicon photoelectrochemical cell for overall water splitting: a natural-artificial photosynthetic hybrid".Angewandte chemie-international edition 55.32(2016):9229-9233. |
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来源:中国科学院大学
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