中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Anaerobic oxidation of methane: geochemical evidence from pore-water in coastal sediments of qi'ao island (pearl river estuary), southern china

文献类型:期刊论文

作者Wu Zijun; Zhou Huaiyang; Peng Xiaotong; Chen Guangqian
刊名Chinese science bulletin
出版日期2006-08-01
卷号51期号:16页码:2006-2015
关键词Anaerobic oxidation of methane (aom) Sulfate-reducing Sediments Pearl river estuary
ISSN号1001-6538
DOI10.1007/s11434-006-2064-6
通讯作者Zhou huaiyang(zhouhy@gig.ac.cn)
英文摘要The concentrations of ch(4) and so(4)(2-) inpore-water and the carbon isotope compositions of total dissolved inorganic (y-co(2)) and ch(4) were determined for three coastal sedimentary cores collected from qi'ao island (pearl river estuary), southern china. results show that methane concentration changes dramatically at the base of the sulfate-reducing zone and sulfate concentration gradients are linear for all stations. in addition, the carbon isotope of methane becomes heavier at the sulfate-methane transition (smt), which causes sigma co(2)-delta(13)c to become the minimum. the geochemical profiles of pore-water render indirect evidence for anaerobic oxidation of methane (aom). based on numerical modeling of aom and sulfate-reducing rates, the portion of total sulfate reduction occurring via aom is 9.0%, 84% and 45.5%, respectively, and the percentage of sigma co(2)added to the pore-water is 4.7%, 72.4% and 29.45% correspondingly for three sites. furthermore, it is found that the methane concentration, methane diffusive flux and the depth of smt are controlled by the quantity and quality of sedimentary organic matter incorporated into the sediments. the great amount of organic material is favorable for rapid depletion of sulfate via sedimentary organic matter degradation, and on the other hand, causes the increase of the methane flux in the smt which results in a portion of sulfate reduction supported by aom. accordingly, the smt was shifted towards the sediment surface.
WOS关键词COUPLED SULFATE REDUCTION ; MARINE-SEDIMENTS ; ORGANIC-MATTER ; SAANICH INLET ; SEA SEDIMENTS ; ACETATE ; RATES ; CONSORTIUM ; PROFILES ; MODEL
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
语种英语
WOS记录号WOS:000241849100014
出版者SCIENCE PRESS
URI标识http://www.irgrid.ac.cn/handle/1471x/2379828
专题中国科学院大学
通讯作者Zhou Huaiyang
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100039, Peoples R China
推荐引用方式
GB/T 7714
Wu Zijun,Zhou Huaiyang,Peng Xiaotong,et al. Anaerobic oxidation of methane: geochemical evidence from pore-water in coastal sediments of qi'ao island (pearl river estuary), southern china[J]. Chinese science bulletin,2006,51(16):2006-2015.
APA Wu Zijun,Zhou Huaiyang,Peng Xiaotong,&Chen Guangqian.(2006).Anaerobic oxidation of methane: geochemical evidence from pore-water in coastal sediments of qi'ao island (pearl river estuary), southern china.Chinese science bulletin,51(16),2006-2015.
MLA Wu Zijun,et al."Anaerobic oxidation of methane: geochemical evidence from pore-water in coastal sediments of qi'ao island (pearl river estuary), southern china".Chinese science bulletin 51.16(2006):2006-2015.

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来源:中国科学院大学

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