Study on ni-re-k/al2o3 catalysts for synthesis of n,n '-di-sec-butyl p-phenylene diamine from p-nitroaniline and 2-butanone
文献类型：期刊论文
| 作者 | Pan, Zhendong; Ding, Yunjie; Jiang, Dahao; Li, Xianming; Jiao, Guiping; Luo, Hongyuan |
| 刊名 | Applied catalysis a-general
 |
| 出版日期 | 2007-10-10 |
| 卷号 | 330页码:43-48 |
| 关键词 | Ni-re-k/al2o3 catalysts N,n '-di-sec-butyl p-phenylene diamine Reductive alkylation Reducibility Surface lewis acidic site |
| ISSN号 | 0926-860X |
| DOI | 10.1016/j.apcata.2007.07.004 |
| 英文摘要 | Ni-re-k/al2o3 catalysts used in reductive alkylation of p-nitroaniline with 2-butanone were investigated by means of bet, xrd, h-2-tpr, nh3-tpd and pyridine-ftir techniques. the results showed that the reducibility and the number of surface lewis acidic sites of the catalysts played a significant role in improving their activities and selectivities. 10ni-1re-1k/al2o3 (gamma-al2o3 calcined at 1173 k) exhibited better reducibility and the proper amount of surface lewis acidic sites, so it performed the highest selectivity towards n,n'-di-sec-butyl p-phenylene diamine among the catalysts. (c) 2007 elsevier b.v. all rights reserved. |
| WOS关键词 | TEMPERATURE-PROGRAMMED-REDUCTION ; THERMAL-STABILITY ; NICKEL-OXIDE ; ALUMINA ; HYDROGENATION ; IMINES |
| WOS研究方向 | Chemistry ; Environmental Sciences & Ecology |
| WOS类目 | Chemistry, Physical ; Environmental Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:000249864300005 |
| 出版者 | ELSEVIER SCIENCE BV |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2380227 |
| 专题 | 中国科学院大学 |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalys, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Pan, Zhendong,Ding, Yunjie,Jiang, Dahao,et al. Study on ni-re-k/al2o3 catalysts for synthesis of n,n '-di-sec-butyl p-phenylene diamine from p-nitroaniline and 2-butanone[J]. Applied catalysis a-general,2007,330:43-48. |
| APA | Pan, Zhendong,Ding, Yunjie,Jiang, Dahao,Li, Xianming,Jiao, Guiping,&Luo, Hongyuan.(2007).Study on ni-re-k/al2o3 catalysts for synthesis of n,n '-di-sec-butyl p-phenylene diamine from p-nitroaniline and 2-butanone.Applied catalysis a-general,330,43-48. |
| MLA | Pan, Zhendong,et al."Study on ni-re-k/al2o3 catalysts for synthesis of n,n '-di-sec-butyl p-phenylene diamine from p-nitroaniline and 2-butanone".Applied catalysis a-general 330(2007):43-48. |
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来源：中国科学院大学
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