Catalytic oxidation of dimethyl ether to dimethoxymethane over cs modified h3pw12o40/sio2 catalysts
文献类型：期刊论文
| 作者 | Zhang, Qingde1,2; Tan, Yisheng1; Yang, Caihong1; Han, Yizhuo1; Shamoto, Jun3; Tsubaki, Noritatsu3 |
| 刊名 | Journal of natural gas chemistry
 |
| 出版日期 | 2007-09-01 |
| 卷号 | 16期号:3页码:322-325 |
| 关键词 | Dimethyl ether Dimethoxymethane Catalytic oxidation Cs modified h3pw12o40/sio2 Xrd |
| ISSN号 | 1003-9953 |
| 通讯作者 | Han, yizhuo(hanyz@sxicc.ac.cn) |
| 英文摘要 | The attractive utilization route for one-step catalytic oxidation of dimethyl ether to dimethoxymethane was successfully carried out over the h3pw12o40(40%)/sio2 catalyst, modified by cs, k, ni, and v. the cs modification of h3pw12o40(40%)/sio2 gave the most promising result of 20% dimethyl ether conversion and 34.8% dimethoxymethane selectivity. dimethoxymethane could be synthesized via methoxy groups decomposed from dimethyl ether through the synergistic effect between the acid sites and the redox sites of cs modified. h3pw12o40(40%)/sio2. |
| WOS关键词 | SUPPORTED HETEROPOLYACID SALTS ; SELECTIVE OXIDATION ; METHANOL ; PERFORMANCE ; METHYLAL |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering |
| WOS类目 | Chemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical |
| 语种 | 英语 |
| WOS记录号 | WOS:000255240200015 |
| 出版者 | ELSEVIER SCIENCE BV |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2380754 |
| 专题 | 中国科学院大学 |
| 通讯作者 | Han, Yizhuo |
| 作者单位 | 1.Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Shanxi, Peoples R China 2.Grad Univ, Chinese Acad Sci, Beijing 100049, Peoples R China 3.Toyama Univ, Dept Appl Chem, Toyama 9308555, Japan |
| 推荐引用方式 GB/T 7714 | Zhang, Qingde,Tan, Yisheng,Yang, Caihong,et al. Catalytic oxidation of dimethyl ether to dimethoxymethane over cs modified h3pw12o40/sio2 catalysts[J]. Journal of natural gas chemistry,2007,16(3):322-325. |
| APA | Zhang, Qingde,Tan, Yisheng,Yang, Caihong,Han, Yizhuo,Shamoto, Jun,&Tsubaki, Noritatsu.(2007).Catalytic oxidation of dimethyl ether to dimethoxymethane over cs modified h3pw12o40/sio2 catalysts.Journal of natural gas chemistry,16(3),322-325. |
| MLA | Zhang, Qingde,et al."Catalytic oxidation of dimethyl ether to dimethoxymethane over cs modified h3pw12o40/sio2 catalysts".Journal of natural gas chemistry 16.3(2007):322-325. |
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来源：中国科学院大学
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