中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Real time and in situ control of the gap size of nanoelectrodes for molecular devices

文献类型:期刊论文

作者Wei, Dacheng1,2; Liu, Yunqi1; Cao, Lingchao1,2; Wang, Yu1,2; Zhang, Hongliang1,2; Yu, Gui1
刊名Nano letters
出版日期2008-06-01
卷号8期号:6页码:1625-1630
ISSN号1530-6984
DOI10.1021/nl080283+
通讯作者Liu, yunqi(liuyq@mail.iccas.ac.cn)
英文摘要Molecular electronics is often limited by the lack of a simple method to fabricate nanoelectrodes with controlled gap size. this is partly attributed to the lack of a real time characterization in the fabrication. here, we report a new method based on an electron induced deposition process operated in scanning electron microscopy that realizes in situ and real time characterization in the nanoelectrode fabrication; thus the gap size can be controlled easily and precisely. it is a clean and nondestructive process for carbon nanotube (cnt) electrodes. the mechanism is detailed. the nanoelectrodes have a pi-conjugated surface due to the deposition of sp(2)-rich amorphous carbon. as an application, dna molecules are assembled between the cnt electrodes by pi-stacking interaction for current-voltage measurement. our result provides a feasible route to prepare nanoelectrodes with controlled gap size, and it will be valuable for current efforts in molecular electronics and nanoelectronics.
WOS关键词WALLED CARBON NANOTUBES ; ON-WIRE LITHOGRAPHY ; ELECTRICAL-TRANSPORT ; AMORPHOUS-CARBON ; RAMAN-SPECTROSCOPY ; BEAM IRRADIATION ; DNA-MOLECULES ; SINGLE ; ADSORPTION ; FILMS
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
语种英语
WOS记录号WOS:000256742000012
出版者AMER CHEMICAL SOC
URI标识http://www.irgrid.ac.cn/handle/1471x/2384390
专题中国科学院大学
通讯作者Liu, Yunqi
作者单位1.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100080, Peoples R China
2.Chinese Acad Sci, Grad Sch, Beijing 100080, Peoples R China
推荐引用方式
GB/T 7714
Wei, Dacheng,Liu, Yunqi,Cao, Lingchao,et al. Real time and in situ control of the gap size of nanoelectrodes for molecular devices[J]. Nano letters,2008,8(6):1625-1630.
APA Wei, Dacheng,Liu, Yunqi,Cao, Lingchao,Wang, Yu,Zhang, Hongliang,&Yu, Gui.(2008).Real time and in situ control of the gap size of nanoelectrodes for molecular devices.Nano letters,8(6),1625-1630.
MLA Wei, Dacheng,et al."Real time and in situ control of the gap size of nanoelectrodes for molecular devices".Nano letters 8.6(2008):1625-1630.

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来源:中国科学院大学

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