A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics
文献类型:期刊论文
| 作者 | Ren, Ze-feng1; Zhou, Chuan-yao1; Ma, Zhi-bo1; Xiao, Chun-lei1; Mao, Xin-chun1; Dai, Dong-xu1; LaRue, Jerry2; Cooper, Russell2; Wodtke, Alec M.2; Yang, Xue-ming1 |
| 刊名 | chinese journal of chemical physics
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| 出版日期 | 2010-06-27 |
| 卷号 | 23期号:3页码:255-261 |
| 关键词 | Femtosecond two-photon photoemission spectropy Time-resolved Ultrafast excited electron dynamics Surface photochemical kinetics |
| 产权排序 | 1;1 |
| 通讯作者 | 杨学明 |
| 英文摘要 | a surface femtosecond two-photon photoemission (2ppe) spectrometer devoted to the study of ultrafast excited electron dynamics and photochemical kinetics on metal and metal oxide surfaces has been constructed. low energy photoelectrons are measured using a hemispherical electron energy analyzer with an imaging detector that allows us to detect the energy and the angular distributions of the photoelectrons simultaneously. a mach-zehnder interferometer was built for the time-resolved 2ppe (tr-2ppe) measurement to study ultrafast surface excited electron dynamics, which was demonstrated on the cu(111) surface. a scheme for measuring time-dependent 2ppe (td-2ppe) spectra has also been developed for studies of surface photochemistry. this technique has been applied to a preliminary study on the photochemical kinetics on ethanol/tio(2)(110). we have also shown that the ultrafast dynamics of photoinduced surface excited resonances can be investigated in a reliable way by combining the tr-2ppe and td-2ppe techniques. |
| WOS标题词 | science & technology ; physical sciences |
| 类目[WOS] | physics, atomic, molecular & chemical |
| 研究领域[WOS] | physics |
| 关键词[WOS] | molecule-metal interfaces ; image-potential states ; resolved photoemission ; energy relaxation ; spectroscopy ; excitation ; cu(111) |
| 收录类别 | SCI |
| 原文出处 | false |
| 语种 | 英语 |
| WOS记录号 | WOS:000280094700003 |
| 公开日期 | 2010-11-30 |
| 源URL | [http://159.226.238.44/handle/321008/103195] ![]() |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 作者单位 | 1.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 2.Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA |
| 推荐引用方式 GB/T 7714 | Ren, Ze-feng,Zhou, Chuan-yao,Ma, Zhi-bo,et al. A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics[J]. chinese journal of chemical physics,2010,23(3):255-261. |
| APA | Ren, Ze-feng.,Zhou, Chuan-yao.,Ma, Zhi-bo.,Xiao, Chun-lei.,Mao, Xin-chun.,...&Yang, Xue-ming.(2010).A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics.chinese journal of chemical physics,23(3),255-261. |
| MLA | Ren, Ze-feng,et al."A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics".chinese journal of chemical physics 23.3(2010):255-261. |
入库方式: OAI收割
来源:大连化学物理研究所
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