Partial oxidation reforming of biomass fuel gas over nickel-based monolithic catalyst with naphthalene as model compound
文献类型：期刊论文
| 作者 | Wang, Chen Guang1,3; Wang, Tie Jun1,2; Ma, Long Long1,2; Gao, Yan1,3; Wu, Chuang Zhi1,2 |
| 刊名 | Korean journal of chemical engineering
 |
| 出版日期 | 2008-07-01 |
| 卷号 | 25期号:4页码:738-743 |
| 关键词 | Biomass fuel gas Monolithic catalyst Partial oxidation reforming Tar elimination |
| ISSN号 | 0256-1115 |
| 通讯作者 | Wang, tie jun(wangtj@ms.giec.ac.cn) |
| 英文摘要 | With naphthalene as biomass tar model compound, partial oxidation reforming (with addition of o-2) and dry reforming of biomass fuel gas were investigated over nickel-based monoliths at the same conditions. the results showed that both processes had excellent performance in upgrading biomass raw fuel gas. above 99% of naphthalene was converted into synthesis gases (h-2+co). about 2.8 wt% of coke deposition was detected on the catalyst surface for dry reforming process at 750 degrees c during 108 h lifetime test. however, no coke deposition was detected for partial oxidation reforming process, which indicated that addition of o-2 can effectively prohibit the coke formation. o-2 can also increase the ch4 conversion and h-2/co ratio of the producer gas. the average conversion of ch4 in dry and partial oxidation reforming process was 92% and 95%, respectively. the average h-2/co ratio increased from 0.95 to 1.1 with the addition of o-2, which was suitable to be used as synthesis gas for dimethyl ether (dme) synthesis. |
| WOS关键词 | FLUIDIZED-BEDS ; NATURAL-GAS ; GASIFICATION ; METHANE ; COMBUSTION ; PERFORMANCE ; ELIMINATION ; NI/AL2O3 ; REACTOR ; SYNGAS |
| WOS研究方向 | Chemistry ; Engineering |
| WOS类目 | Chemistry, Multidisciplinary ; Engineering, Chemical |
| 语种 | 英语 |
| WOS记录号 | WOS:000258549600019 |
| 出版者 | KOREAN INST CHEM ENGINEERS |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2390987 |
| 专题 | 中国科学院大学 |
| 通讯作者 | Wang, Tie Jun |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China 3.Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Chen Guang,Wang, Tie Jun,Ma, Long Long,et al. Partial oxidation reforming of biomass fuel gas over nickel-based monolithic catalyst with naphthalene as model compound[J]. Korean journal of chemical engineering,2008,25(4):738-743. |
| APA | Wang, Chen Guang,Wang, Tie Jun,Ma, Long Long,Gao, Yan,&Wu, Chuang Zhi.(2008).Partial oxidation reforming of biomass fuel gas over nickel-based monolithic catalyst with naphthalene as model compound.Korean journal of chemical engineering,25(4),738-743. |
| MLA | Wang, Chen Guang,et al."Partial oxidation reforming of biomass fuel gas over nickel-based monolithic catalyst with naphthalene as model compound".Korean journal of chemical engineering 25.4(2008):738-743. |
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来源：中国科学院大学
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