Electrolysis and heat pretreatment methods to promote co(2) sequestration by mineral carbonation
文献类型：期刊论文
| 作者 | Li, Wenzhi1,2; Li, Wen1; Lia, Baoqing1; Bai, Zongqing1 |
| 刊名 | Chemical engineering research & design
 |
| 出版日期 | 2009-02-01 |
| 卷号 | 87期号:2a页码:210-215 |
| 关键词 | Electrolysis Co(2) sequestration Mineral carbonation Serpentine Heat pretreatment |
| ISSN号 | 0263-8762 |
| DOI | 10.1016/j.cherd.2008.08.001 |
| 通讯作者 | Li, wenzhi(liwen@sxicc.ac.cn) |
| 英文摘要 | As a new mineral carbonation process for co(2) sequestration, electrolysis of nacl solution and serpentine as the source of me(2+) to adsorb co(2) in the simulating flue gas is introduced, which used the electrolyze nacl solution to produce the hcl solution and naoh solution. the hcl solution was used to dissolve me(2+) from serpentine, and the naoh solution was used to adsorb co(2) in simulation smoke, then these two solutions were mixed to form mgco(3) deposition at 358 k, which could be processed at relative low temperature and pressure. in order to further increase the solubility of me(2+) from serpentine, the heat pretreatment of serpentine under nitrogen was investigated. the results indicated that the heat activation dramatically enhanced serpentine carbonation. xrd, tga, ft-ir and icp-aes analyses indicated that the best activation temperature was 650 degrees c, at which the crystalline features were changed from lizardite to amorphous followed the decomposition of hydroxyl groups. the dissolved capacity decreased with further increasing heat activation temperature, which might be related to the formation of a new crystalline feature. the xrd and tga analyses showed that the solid product was mainly pure basic magnesium carbonate. (c) 2008 the institution of chemical engineers. published by elsevier b.v. all rights reserved. |
| WOS关键词 | SERPENTINE ; ACTIVATION ; STORAGE ; BRINE ; PH |
| WOS研究方向 | Engineering |
| WOS类目 | Engineering, Chemical |
| 语种 | 英语 |
| WOS记录号 | WOS:000263639800009 |
| 出版者 | INST CHEMICAL ENGINEERS |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2404699 |
| 专题 | 中国科学院大学 |
| 通讯作者 | Li, Wenzhi |
| 作者单位 | 1.Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, Taiyuan 030001, Shanxi, Peoples R China 2.Chinese Acad Sci, Grad Sch, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Wenzhi,Li, Wen,Lia, Baoqing,et al. Electrolysis and heat pretreatment methods to promote co(2) sequestration by mineral carbonation[J]. Chemical engineering research & design,2009,87(2a):210-215. |
| APA | Li, Wenzhi,Li, Wen,Lia, Baoqing,&Bai, Zongqing.(2009).Electrolysis and heat pretreatment methods to promote co(2) sequestration by mineral carbonation.Chemical engineering research & design,87(2a),210-215. |
| MLA | Li, Wenzhi,et al."Electrolysis and heat pretreatment methods to promote co(2) sequestration by mineral carbonation".Chemical engineering research & design 87.2a(2009):210-215. |
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来源：中国科学院大学
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