Synthesis of highly nitrogen-doped hollow carbon nanoparticles and their excellent electrocatalytic properties in dye-sensitized solar cells
文献类型：期刊论文
| 作者 | Jia, Rongrong1,2; Chen, Jiazang1,2; Zhao, Jianghong1; Zheng, Jianfeng1; Song, Chang1; Li, Li1; Zhu, Zhenping1 |
| 刊名 | Journal of materials chemistry
 |
| 出版日期 | 2010 |
| 卷号 | 20期号:48页码:10829-10834 |
| ISSN号 | 0959-9428 |
| DOI | 10.1039/c0jm01799j |
| 通讯作者 | Zhao, jianghong(zjh_sx@sxicc.ac.cn) |
| 英文摘要 | Hollow carbon nanoparticles that have been highly doped with nitrogen (n-hcnps) are directly prepared by a facile one-pot method based on the detonation-assisted chemical vapor deposition of dimethylformamide without the use of metal catalysts. the n-hcnps exhibit uniform core-shell microstructures with inner cavities encapsulated by graphitic walls, possessing a narrow size distribution of 10-25 nm. the nitrogen content in n-hcnps is as high as 20.8% atom ratio, and the nitrogen bonds display pyridine-, pyrrole-, and graphite-like configurations. defects and dislocations are present in the graphene layers due to highly incorporated nitrogen, leading to the creation of micropores on the carbon shell and a large bet surface area of 454 m(2) g(-1). the unique n-hcnps with interconnected hierarchical porous structures and nitrogen-containing defects show excellent electrocatalytic activity for triiodide reduction in dye-sensitized solar cells, superior to conventional platinum catalysts. |
| WOS关键词 | OXYGEN REDUCTION ; COUNTER ELECTRODES ; NANOTUBES ; FILMS ; GROWTH ; PYROLYSIS ; HYDROGENATION ; DETONATION ; GRAPHITE ; GRAPHENE |
| WOS研究方向 | Chemistry ; Materials Science |
| WOS类目 | Chemistry, Physical ; Materials Science, Multidisciplinary |
| 语种 | 英语 |
| WOS记录号 | WOS:000284773100009 |
| 出版者 | ROYAL SOC CHEMISTRY |
| URI标识 | http://www.irgrid.ac.cn/handle/1471x/2405465 |
| 专题 | 中国科学院大学 |
| 通讯作者 | Zhao, Jianghong |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Coal Convers, Inst Coal Chem, Taiyuan 030001, Peoples R China 2.Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jia, Rongrong,Chen, Jiazang,Zhao, Jianghong,et al. Synthesis of highly nitrogen-doped hollow carbon nanoparticles and their excellent electrocatalytic properties in dye-sensitized solar cells[J]. Journal of materials chemistry,2010,20(48):10829-10834. |
| APA | Jia, Rongrong.,Chen, Jiazang.,Zhao, Jianghong.,Zheng, Jianfeng.,Song, Chang.,...&Zhu, Zhenping.(2010).Synthesis of highly nitrogen-doped hollow carbon nanoparticles and their excellent electrocatalytic properties in dye-sensitized solar cells.Journal of materials chemistry,20(48),10829-10834. |
| MLA | Jia, Rongrong,et al."Synthesis of highly nitrogen-doped hollow carbon nanoparticles and their excellent electrocatalytic properties in dye-sensitized solar cells".Journal of materials chemistry 20.48(2010):10829-10834. |
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来源：中国科学院大学
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