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Optical properties of nanotube bundles by photoluminescence excitation and absorption spectroscopy

文献类型:期刊论文

作者Tan, P. H.1,2; Hasan, T.1; Bonaccorso, F.1,3; Scardaci, V.1; Rozhin, A. G.1; Milne, W. I.1; Ferrari, A. C.1
刊名Physica e-low-dimensional systems & nanostructures
出版日期2008-05-01
卷号40期号:7页码:2352-2359
关键词Photoluminescence excitation Absorption Bundle Carbon nanotube
ISSN号1386-9477
DOI10.1016/j.physe.2007.10.058
通讯作者Tan, p. h.(pt290@eng.cam.ac.uk)
英文摘要Photoluminescence excitation (ple) and absorption spectroscopy are applied to investigate the impact of bundle size on the optical properties of single wall carbon nanotube (swnt) bundles in aqueous suspensions. the existence and gradual formation of small bundles happens in aqueous suspensions even after ultrasonication and ultracentrifugation. with time, the emission and absorption spectra show weaker intensities and broader spectral profiles, confirming the formation of bigger saint bundles. we detect new ple features assigned to energy transfer from excitons and excitonic phonon sidebands of donors to eh(11) excitons of acceptors in such suspensions. in addition, the photoluminescence intensity from large gap nanotube donors weakens, while that from the smaller gap acceptors increases because of the exciton energy transfer. our results caution the use of photoluminescence to determine the abundance of different swnt species in conventionally prepared aqueous suspensions. on the contrary, absorption measurements represent a more reliable technique to reveal such information. (c) 2007 elsevier b.v. all rights reserved.
WOS关键词WALLED CARBON NANOTUBES
WOS研究方向Science & Technology - Other Topics ; Physics
WOS类目Nanoscience & Nanotechnology ; Physics, Condensed Matter
语种英语
WOS记录号WOS:000257186500027
出版者ELSEVIER SCIENCE BV
URI标识http://www.irgrid.ac.cn/handle/1471x/2427450
专题半导体研究所
通讯作者Tan, P. H.
作者单位1.Univ Cambridge, Dept Engn, Cambridge CB3 0FA, England
2.State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China
3.Univ Messina, CNR, Ist Proc Chim Fis, I-98166 Messina, Italy
4.Univ Messina, Dept Fis Mat & Tecnol Fis Avanzate, I-98166 Messina, Italy
推荐引用方式
GB/T 7714
Tan, P. H.,Hasan, T.,Bonaccorso, F.,et al. Optical properties of nanotube bundles by photoluminescence excitation and absorption spectroscopy[J]. Physica e-low-dimensional systems & nanostructures,2008,40(7):2352-2359.
APA Tan, P. H..,Hasan, T..,Bonaccorso, F..,Scardaci, V..,Rozhin, A. G..,...&Ferrari, A. C..(2008).Optical properties of nanotube bundles by photoluminescence excitation and absorption spectroscopy.Physica e-low-dimensional systems & nanostructures,40(7),2352-2359.
MLA Tan, P. H.,et al."Optical properties of nanotube bundles by photoluminescence excitation and absorption spectroscopy".Physica e-low-dimensional systems & nanostructures 40.7(2008):2352-2359.

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来源:半导体研究所

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