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Influence of zns and mgo shell on the photoluminescence properties of zno core/shell nanowires

文献类型:期刊论文

作者Meng, X. Q.; Peng, Haowei; Gai, Y. Q.; Li, Jingbo
刊名Journal of physical chemistry c
出版日期2010-01-28
卷号114期号:3页码:1467-1471
ISSN号1932-7447
DOI10.1021/jp909176p
通讯作者Li, jingbo(jbli@semi.ac.cn)
英文摘要By sequential growth of the core and shell of different materials, zno/zns and zno/mgo core/shell nanowire arrays are fabricated. photoluminescence properties of these samples with different shell thicknesses are studied in detail. the results indicate that the zns shell thickness as a function of treatment time will noticeably change the photoluminescence intensity of the zno nanowires, whereas the mgo shell will not change the photoluminescence intensity any more after it saturates the surface dangling bonds of zno core. large-scale first-principles calculations indicate that, unlike the zno/mgo core/shell nanowires, the electrons and holes of which are both confined in the core of the nanowires (type-i heterostructures), the zno/zns core/shell nanowires are type-ii heterostructures, the electrons and holes of which are respectively confined in the core and the shell; as a result, the separation of electrons and holes in the zno/zns core/shell nanowires will reduce the spatial overlap between them, leading to the decrease of the photoluminescence intensity in this system. the experimental observations are in good agreement with first-principles calculations
WOS关键词COLLOIDAL NANOCRYSTAL HETEROSTRUCTURES ; OPTICAL-PROPERTIES ; NANOSTRUCTURES ; NANORODS ; DOTS
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
WOS类目Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
语种英语
WOS记录号WOS:000273672500011
出版者AMER CHEMICAL SOC
URI标识http://www.irgrid.ac.cn/handle/1471x/2427889
专题半导体研究所
通讯作者Li, Jingbo
作者单位Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, Beijing 100083, Peoples R China
推荐引用方式
GB/T 7714
Meng, X. Q.,Peng, Haowei,Gai, Y. Q.,et al. Influence of zns and mgo shell on the photoluminescence properties of zno core/shell nanowires[J]. Journal of physical chemistry c,2010,114(3):1467-1471.
APA Meng, X. Q.,Peng, Haowei,Gai, Y. Q.,&Li, Jingbo.(2010).Influence of zns and mgo shell on the photoluminescence properties of zno core/shell nanowires.Journal of physical chemistry c,114(3),1467-1471.
MLA Meng, X. Q.,et al."Influence of zns and mgo shell on the photoluminescence properties of zno core/shell nanowires".Journal of physical chemistry c 114.3(2010):1467-1471.

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来源:半导体研究所

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