Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition
文献类型：期刊论文
| 作者 | Gao, Wenbo1,2; Guo, Jianping2,3; Chen, Ping2,3 |
| 刊名 | CHINESE JOURNAL OF CHEMISTRY
 |
| 出版日期 | 2019-05-01 |
| 卷号 | 37期号:5页码:442-451 |
| ISSN号 | 1001-604X |
| 关键词 | ammonia synthesis ammonia decomposition hydride imide amide |
| DOI | 10.1002/cjoc.201800586 |
| 通讯作者 | Guo, Jianping(guojianping@dicp.ac.cn) ; Chen, Ping(pchen@dicp.ac.cn) |
| 英文摘要 | Ammonia is feeding nearly half the world population and also holds the promise as a carbon-free energy carrier. The development of ammonia synthesis and decomposition processes under milder conditions is a grand challenge for more than a century. Increasing effort is devoted to this area in recent years and encouraging progress has been achieved. In this paper, we summarize our recent research using alkali or alkaline earth metal amides, imides and hydrides for ammonia synthesis and decomposition. These materials could serve as either indispensible component of active center in thermal catalytic process or nitrogen carrier for chemical looping ammonia synthesis. The synergy of amide, imide, or hydride with transition metals enables ammonia synthesis or decomposition with unprecedented high efficiency under milder reaction conditions, and thus opens an avenue to advance the chemistry or catalysis of N-2 fixation reaction. The compositional and structural diversity of the amide, imide and hydride materials provides plenty of opportunity and potential for further exploration and optimization. |
| WOS关键词 | METAL NITRIDES ; MANGANESE NITRIDE ; NITROGEN TRANSFER ; HYDROGEN STORAGE ; CATALYSTS ; NH3 ; EFFICIENT ; N-2 ; RU ; GENERATION |
| 资助项目 | National Natural Science Foundation of China[21633011] ; National Natural Science Foundation of China[21603220] ; National Natural Science Foundation of China[21872137] ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology[2016YFE0118300] ; DICP[DICP DMTO201504] ; Youth Innovation Promotion Association CAS[2018213] ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000466442600002 |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/165526]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Guo, Jianping; Chen, Ping |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China 3.Collaborat Innovat Ctr Chem Energy Mat, Dalian 116023, Liaoning, Peoples R China |
| 推荐引用方式 GB/T 7714 | Gao, Wenbo,Guo, Jianping,Chen, Ping. Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition[J]. CHINESE JOURNAL OF CHEMISTRY,2019,37(5):442-451. |
| APA | Gao, Wenbo,Guo, Jianping,&Chen, Ping.(2019).Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition.CHINESE JOURNAL OF CHEMISTRY,37(5),442-451. |
| MLA | Gao, Wenbo,et al."Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition".CHINESE JOURNAL OF CHEMISTRY 37.5(2019):442-451. |
入库方式： OAI收割
来源：大连化学物理研究所
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