Investigation on the reaction area of PEMFC at different position in multiple catalyst layer
文献类型：期刊论文
| 作者 | Lin, Rui1; Li, Wenbin1; Yang, Yue2 |
| 刊名 | ELECTROCHIMICA ACTA
 |
| 出版日期 | 2019-04-10 |
| 卷号 | 302页码:241-248 |
| 关键词 | PEMFC Multiple catalyst layer EIS Performance |
| ISSN号 | 0013-4686 |
| DOI | 10.1016/j.electacta.2019.02.003 |
| 通讯作者 | Lin, Rui(ruilin@tongji.edu.cn) |
| 英文摘要 | To study the oxygen reduction reaction (ORR) at different through-plane position in catalyst layer, a multiple catalyst layer (MCL) was designed in which the reaction area could move from proton exchange membrane (PEM) to gas diffusion layer (GDL). The reaction layer (layer Y) was sandwiched between proton conduct layer (layer X) and air diffusion layer (layer Z) to simulate the real reacting process in an ordinary catalyst layer. Three MEA samples with MCL were made, the reaction area was set near the PEM, in the middle of catalyst layer and near the GDL, respectively. According to the polarization curves, the position of reaction area in catalyst layer has obvious influence on cell performance and the output current at the same working voltage increased when the reaction area moved towards GDL. Besides, how the charge transfer resistance and mass transport resistance of reaction area at different position in CL changed when output current increased has also been studied in this work using EIS. Simulation results about current and proton distribution have also been verified in this work. (C) 2019 Elsevier Ltd. All rights reserved. |
| WOS关键词 | MEMBRANE FUEL-CELL ; PERFORMANCE ; ELECTRODE ; GRADIENT ; CONDUCTIVITY ; IMPROVEMENT ; CATHODE ; INK |
| 资助项目 | National Natural Science Foundation of China[21776222] ; National Key Research and Development Program of China[2017YFB0102803] |
| WOS研究方向 | Electrochemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000459998000027 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/165866]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Lin, Rui |
| 作者单位 | 1.Tongji Univ, Sch Automot Studies, 4800 Caoan Rd, Shanghai 201804, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Fuel Cell Syst & Engn Lab, 457 Zhongshan Rd, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lin, Rui,Li, Wenbin,Yang, Yue. Investigation on the reaction area of PEMFC at different position in multiple catalyst layer[J]. ELECTROCHIMICA ACTA,2019,302:241-248. |
| APA | Lin, Rui,Li, Wenbin,&Yang, Yue.(2019).Investigation on the reaction area of PEMFC at different position in multiple catalyst layer.ELECTROCHIMICA ACTA,302,241-248. |
| MLA | Lin, Rui,et al."Investigation on the reaction area of PEMFC at different position in multiple catalyst layer".ELECTROCHIMICA ACTA 302(2019):241-248. |
入库方式： OAI收割
来源：大连化学物理研究所
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