中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Mosquito's Compound Eyes as Inspiration for Fabrication of Conductive Superhydrophobic Nanocarbon Materials from Waste Wheat Straw

文献类型:期刊论文

作者Su, Qiong1,2; Wang, Yanbin1,2; Zhang, Dong1,2; Deng, June3; Zhou, Feng4; Duan, Zhiying1,2; Pang, Shaofeng1,2
刊名ACS SUSTAINABLE CHEMISTRY & ENGINEERING
出版日期2019-02-18
卷号7期号:4页码:3883-3894
关键词Biomimetic Wheat straw Controllable construction Superhydrophobicity Conductivity Nanocarbon materials
ISSN号2168-0485
DOI10.1021/acssuschemeng.8b04906
通讯作者Su, Qiong(hgsq@xbmu.edu.cn) ; Pang, Shaofeng(pangshaofeng2006@163.com)
英文摘要Converting waste wheat straw to conductive superhydrophobic nanocarbon materials is inspired by mosquitos compound eyes, and a one step pyrolysis process is used for controllable construction of micro/nanohierarchical structures. Their structures and hydrophobicity can be tuned efficiently by the annealing temperature. Scanning electron microscopy, elemental analysis, X-ray diffraction, laser Raman, Fourier transform infrared, and photoelectron spectroscopy analyses were used to reveal the structure of electrical conductive carbon materials (ECMs) and a possible mechanism of the nanostructures formation. These results indicate that there are big differences between the surface and the inner structure for the nanocarbon materials, and the releasing rates of a multicomponent gas at different annealing temperatures by further decomposition of waste wheat straw should be pivotal to the formation of nanostructures. There is also cause for superhydrophobicity and electroconductivity for the ECM-800. Considering the potential use of the novel ECM-800, a low-cost, green, sustainable, conductive, and superhydrophobic coating strategy was developed by dip-coating of the different substrates with a ECM-800/PDMS mixture, followed by thermal curing. The water contact angle of the prepared ECM-800/PDMS coating is greater than 160 degrees, while the sliding angle is less than 5 degrees, showing excellent superhydrophobicity as well as good mechanical robustness and water-repellency in the artificial rain tests simultaneously. In addition, a robust ECM-800 enables resistance to a variety of harsh environments, such as an ability to resist heat and UV aging as well as sustaining exposure to strong acid/alkaline corrosion. Moreover, this work should be conducive to the controllable construction of conductive superhydrophobic nanocarbon materials with well-defined structure, and open up a convenient sustainable way for disposal of waste biomass for production of value-added materials.
WOS关键词GRAPHENE OXIDE ; WETTABILITY TRANSITION ; CARBONACEOUS MATERIALS ; GOLD SURFACES ; HIGH-PRESSURE ; LARGE-SCALE ; BIOMASS ; BIOCHARS ; OXYGEN ; SPECTROSCOPY
资助项目National Natural Science Foundation of China[51563022] ; Fundamental Research Funds for the Central Universities[1001050227] ; Scientific Research Foundation of Northwest University for Nationalities[xbmuyjrc 201705]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Engineering
语种英语
WOS记录号WOS:000459367400027
出版者AMER CHEMICAL SOC
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Scientific Research Foundation of Northwest University for Nationalities ; Scientific Research Foundation of Northwest University for Nationalities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Scientific Research Foundation of Northwest University for Nationalities ; Scientific Research Foundation of Northwest University for Nationalities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Scientific Research Foundation of Northwest University for Nationalities ; Scientific Research Foundation of Northwest University for Nationalities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; Scientific Research Foundation of Northwest University for Nationalities ; Scientific Research Foundation of Northwest University for Nationalities
源URL[http://cas-ir.dicp.ac.cn/handle/321008/165898]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Su, Qiong; Pang, Shaofeng
作者单位1.Northwest Minzu Univ, Chem Engn Inst, 1 Northwest Xincun, Lanzhou 730030, Gansu, Peoples R China
2.Northwest Minzu Univ, Key Lab Environm Friendly Composite Mat & Biomass, 1 Northwest Xincun, Lanzhou 730030, Gansu, Peoples R China
3.Northwest Minzu Univ, Sch Foreign Languages, 1 Northwest Xincun, Lanzhou 730030, Gansu, Peoples R China
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
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GB/T 7714
Su, Qiong,Wang, Yanbin,Zhang, Dong,et al. Mosquito's Compound Eyes as Inspiration for Fabrication of Conductive Superhydrophobic Nanocarbon Materials from Waste Wheat Straw[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2019,7(4):3883-3894.
APA Su, Qiong.,Wang, Yanbin.,Zhang, Dong.,Deng, June.,Zhou, Feng.,...&Pang, Shaofeng.(2019).Mosquito's Compound Eyes as Inspiration for Fabrication of Conductive Superhydrophobic Nanocarbon Materials from Waste Wheat Straw.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,7(4),3883-3894.
MLA Su, Qiong,et al."Mosquito's Compound Eyes as Inspiration for Fabrication of Conductive Superhydrophobic Nanocarbon Materials from Waste Wheat Straw".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 7.4(2019):3883-3894.

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来源:大连化学物理研究所

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