Antifouling behavior on the linear suspension PEG-based surface and two-end-linked PEG-based surface of composite nanofiltration membranes via two-step interfacial polymerization
文献类型:期刊论文
作者 | Kang, Te3; Wang, Qi1,2; Kang, Guodong4; Zhao, Hongyong1,2; Ding, Xiaoli1,2; Zhang, Yuzhong1,2 |
刊名 | DESALINATION AND WATER TREATMENT
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出版日期 | 2019-03-01 |
卷号 | 144页码:9-25 |
关键词 | Antifouling Poly(ethylene glycol) based Linear suspension Two-end-linked Two-step interfacial polymerization |
ISSN号 | 1944-3994 |
DOI | 10.5004/dwt.2019.23504 |
通讯作者 | Zhao, Hongyong(zhaohongyong@tjpu.edu.cn) |
英文摘要 | Hydrophilic nanofiltration membranes with single-layered or double-layered poly(ethylene glycol) (PEG) based structure were fabricated by two-step interfacial polymerization (IP) to enhance antifouling property. O,O'-bis(2-aminopropyl) polypropylene glycol-block-polyethylene glycol-block-polypropylene glycol (jeffamine) was used as monomer and modifier in both layers. The antifouling performance against bovine serum albumin (BSA) for the nascent polyamide membrane with single PEG-based layer was not satisfactory with a highest water flux recovery ratio (FRR) of 75.9%. Therefore, a second IP was performed between jeffamine and the residual unreacted chloroformyl group in selective layer to form an additional PEG-based layer, which demonstrated the two-end-linked structure when jeffamine 2003 was used and the linear suspension structure when jeffamine 600 was used. The results showed that the flux and rejection of membranes with double-layered PEG-based structure had little variation compared with that of single-layered membranes, while the antifouling performance against BSA was significantly improved by the additional PEG-based layer. Moreover, the additional linear suspension PEG-based layer contributed more to antifouling performance than the additional two-end-linked PEG-based structure. The membrane with the additional linear suspension PEG-based layer displayed a highest water FRR of 99.6%, while the membrane with the additional two-end-linked PEG-based layer displayed a highest water FRR of 83.6%. |
WOS关键词 | THIN-FILM COMPOSITE ; IN-SITU PEGYLATION ; OSMOSIS MEMBRANES ; REVERSE-OSMOSIS ; NANOCOMPOSITE MEMBRANE ; WATER ; FABRICATION |
资助项目 | National Natural Science Foundation of China[21776217] ; Technology Plans of Tianjin[17PTSYJC00050] ; Technology Plans of Tianjin[18PTSYJC 00190] |
WOS研究方向 | Engineering ; Water Resources |
语种 | 英语 |
WOS记录号 | WOS:000458909900002 |
出版者 | DESALINATION PUBL |
资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; Technology Plans of Tianjin ; Technology Plans of Tianjin ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Technology Plans of Tianjin ; Technology Plans of Tianjin ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Technology Plans of Tianjin ; Technology Plans of Tianjin ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Technology Plans of Tianjin ; Technology Plans of Tianjin |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/166020] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Zhao, Hongyong |
作者单位 | 1.Tianjin Polytech Univ, Natl Ctr Int Joint Res Separat Membranes, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China 2.Tianjin Polytech Univ, Tianjin Key Lab Hollow Fiber Membrane Mat & Proc, Tianjin 300387, Peoples R China 3.Beijing Origin Water Technol Co Ltd, Beijing 102206, Peoples R China 4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Kang, Te,Wang, Qi,Kang, Guodong,et al. Antifouling behavior on the linear suspension PEG-based surface and two-end-linked PEG-based surface of composite nanofiltration membranes via two-step interfacial polymerization[J]. DESALINATION AND WATER TREATMENT,2019,144:9-25. |
APA | Kang, Te,Wang, Qi,Kang, Guodong,Zhao, Hongyong,Ding, Xiaoli,&Zhang, Yuzhong.(2019).Antifouling behavior on the linear suspension PEG-based surface and two-end-linked PEG-based surface of composite nanofiltration membranes via two-step interfacial polymerization.DESALINATION AND WATER TREATMENT,144,9-25. |
MLA | Kang, Te,et al."Antifouling behavior on the linear suspension PEG-based surface and two-end-linked PEG-based surface of composite nanofiltration membranes via two-step interfacial polymerization".DESALINATION AND WATER TREATMENT 144(2019):9-25. |
入库方式: OAI收割
来源:大连化学物理研究所
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