Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry
文献类型：期刊论文
| 作者 | Ma, Lei1; Jin, Chengyu2,3; An, Luyang4; Huang, Long1; Li, Linjun1; Jin, Haibo1; Liang, Bo1; Wei, Huangzhao2; Sun, Chenglin2 |
| 刊名 | CATALYSIS COMMUNICATIONS
 |
| 出版日期 | 2019-02-01 |
| 卷号 | 120页码:59-65 |
| 关键词 | Advanced oxidation Sludge-derived carbon nanosheets Quantum chemical calculation Cresols |
| ISSN号 | 1566-7367 |
| DOI | 10.1016/j.catcom.2018.11.012 |
| 通讯作者 | Wei, Huangzhao(whzhdicpwtg@dicp.ac.cn) ; Sun, Chenglin(clsun@dicp.ac.cn) |
| 英文摘要 | Advanced oxidation technology is widely used to oxidize organic compounds in the liquid phase by OH conventionally. Here, we prepared a sludge-derived carbon nanosheets, which was applied in the catalytic wet air oxidation (CWAO), catalytic wet peroxide oxidation (CWPO) and catalytic wet ozone oxidation (CWOO) systems. Because of its abundant oxygen-containing functional groups, the catalytic activity of nanosheets was much higher than some conventional catalysts. It was found that the first-order reaction model did not have similar characteristics as expected. Combining with molecular descriptors calculated by the DFT method and PLS analysis, we try to explain this phenomenon for the first time and proposed possible mechanisms for the three advanced oxidation technologies. |
| WOS关键词 | WET PEROXIDE OXIDATION ; AIR OXIDATION ; ELECTROCHEMICAL DEGRADATION ; WASTE-WATER ; TEMPERATURE ; PHENOL ; ADSORPTION ; KINETICS ; XPS |
| 资助项目 | Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality)[IDHT20180508] ; National Natural Science Foundation of China[51878643] ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology[BZ041420180003] ; DICP[ZZBS201614] ; Beijing undergraduate Research Training Program[2018J00003] ; Beijing undergraduate Research Training Program[2018J00004] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000458222300013 |
| 出版者 | ELSEVIER SCIENCE BV |
| 资助机构 | Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; DICP ; DICP ; Beijing undergraduate Research Training Program ; Beijing undergraduate Research Training Program ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; DICP ; DICP ; Beijing undergraduate Research Training Program ; Beijing undergraduate Research Training Program ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; DICP ; DICP ; Beijing undergraduate Research Training Program ; Beijing undergraduate Research Training Program ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges (under Beijing Municipality) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; special fund of Beijing Key Laboratory of Clean Fuels and Efficient Catalytic Emission Reduction Technology ; DICP ; DICP ; Beijing undergraduate Research Training Program ; Beijing undergraduate Research Training Program |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/166086]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Wei, Huangzhao; Sun, Chenglin |
| 作者单位 | 1.Beijing Inst Petrochem Technol, Beijing Key Lab Fuels Cleaning & Adv Catalyt Emis, Coll Chem Engn, Beijing 102617, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Sinosteel Anshan Res Inst Thermoenergy Co Ltd, Natl Engn Res Ctr Coking Technol, Anshan 114044, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ma, Lei,Jin, Chengyu,An, Luyang,et al. Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry[J]. CATALYSIS COMMUNICATIONS,2019,120:59-65. |
| APA | Ma, Lei.,Jin, Chengyu.,An, Luyang.,Huang, Long.,Li, Linjun.,...&Sun, Chenglin.(2019).Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry.CATALYSIS COMMUNICATIONS,120,59-65. |
| MLA | Ma, Lei,et al."Preliminary investigation of the degradation mechanism of o, m and p-cresol using sludge-derived carbon nanosheets by catalytic oxidation based on quantum chemistry".CATALYSIS COMMUNICATIONS 120(2019):59-65. |
入库方式： OAI收割
来源：大连化学物理研究所
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