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Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses

文献类型：期刊论文

作者Ding, Dajun2; Sun, Zhigang1; Yuan, Kai-Jun2,3; Bandrauk, Andre D.3; Hu, Wenhui2; Liu, Yong1; Luo, Sizuo2; Li, Xing2; Yu, Jiaqi2; Li, Xiaokai2
刊名PHYSICAL REVIEW A
出版日期2019-01-22
卷号99期号:1页码:6
ISSN号2469-9926
DOI10.1103/PhysRevA.99.011402
通讯作者Luo, Sizuo(luosz@jlu.edu.cn) ; Yuan, Kai-Jun(kaijun.yuan@usherbrooke.ca) ; Ding, Dajun(dajund@jlu.edu.cn)
英文摘要Quantum coherence interference between electronic states in molecules is an important factor for controlling electronic and nuclear dynamics in photoinduced physics and chemistry. We measure and model molecular angle-dependent photoionization yields to explore coherent interference dynamics between quasiequal energy electronic-vibrational states of the nitric oxide molecule, NO, by ultrafast phase-controlled two-color femtosecond laser pulses. We demonstrate by experiment and theory that the photoelectron angular distribution of NO, where two excited electronic states are coherently combined by ultrafast pulses, is a function of the relative phase of the pulses, and the photoelectron kinetic energy. The modification of photoelectron emission angular patterns encodes the information of the coherence via electronic state interference. The result allows access to phase-dependent state correlations and ultrafast vibrationic dynamics in molecules.
WOS关键词CIRCULAR-DICHROISM ; DYNAMICS ; PHOTOELECTRON ; DIFFRACTION ; IONIZATION ; MIGRATION ; BREAKING
资助项目National Natural Science Foundation of China (NNSFC)[11704148] ; National Natural Science Foundation of China (NNSFC)[11534004] ; National Natural Science Foundation of China (NNSFC)[11627807] ; National Natural Science Foundation of China (NNSFC)[21222308] ; National Natural Science Foundation of China (NNSFC)[21133006] ; National Natural Science Foundation of China (NNSFC)[21433009] ; China Postdoctoral Science Foundation[2015M571336] ; NSERC ; FQRNT
WOS研究方向Optics ; Physics
语种英语
WOS记录号WOS:000456287500003
出版者AMER PHYSICAL SOC
资助机构National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT
源URL[http://cas-ir.dicp.ac.cn/handle/321008/166292]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Ding, Dajun; Yuan, Kai-Jun; Luo, Sizuo
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Jilin, Peoples R China
3.Univ Sherbrooke, Fac Sci, Lab Chim Theor, Sherbrooke, PQ J1K 2R1, Canada
推荐引用方式
GB/T 7714		 Ding, Dajun,Sun, Zhigang,Yuan, Kai-Jun,et al. Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses[J]. PHYSICAL REVIEW A,2019,99(1):6.
APA Ding, Dajun.,Sun, Zhigang.,Yuan, Kai-Jun.,Bandrauk, Andre D..,Hu, Wenhui.,...&Li, Xiaokai.(2019).Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses.PHYSICAL REVIEW A,99(1),6.
MLA Ding, Dajun,et al."Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses".PHYSICAL REVIEW A 99.1(2019):6.

入库方式： OAI收割

来源：大连化学物理研究所

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