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Graphdiyne as a Host Active Material for Perovskite Solar Cell Application

文献类型：期刊论文

作者Li, Yuliang2,4; Li, Jiangsheng3; Jiu, Tonggang3,4,6; Chen, Siqi3; Liu, Le3; Yao, Quantong3; Bi, Fuzhen3; Zhao, Chengjie3; Wang, Zhen3; Zhao, Min3
刊名NANO LETTERS
出版日期2018-11-01
卷号18期号:11页码:6941-6947
ISSN号1530-6984
关键词Graphdiyne host active material MAPbI(3) perovskite device solar cells
DOI10.1021/acs.nanolett.8b02863
通讯作者Jiu, Tonggang(jiutg@qibebt.ac.cn) ; Li, Yuliang(ylli@iccas.ac.cn)
英文摘要This work demonstrates a novel photovoltaic application in which graphdiyne (GD) can be employed as a host material in a perovskite active layer for the first time. In the device fabrication, the best molar ratio for active materials is verified as PbI2/MAI/GD being 1:1:0.25, yielding a peak power-conversion efficiency of 21.01%. We find that graphdiyne, as the host material, exerts significant influence on the crystallization, film morphology, and a series of optoelectronic properties of the perovskite active layer. A uniform MAPbI(3) film with highly crystalline qualities, large domain sizes, and few grain boundaries was realized with the introduction of graphdiyne. Moreover, the current-voltage hysteresis was negligible, and device stability was significantly improved as well. The results indicate that graphdiyne as the host active material presents great potential for the enhancement of the performance of perovskite solar cells.
WOS关键词ELECTRON-TRANSPORT ; 2D GRAPHDIYNE ; EFFICIENT ; EXTRACTION
资助项目Major Program of Shandong Province Natural Science Foundation[ZR2017ZB0313] ; National Natural Science Foundation of China[51672288] ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT[UN201705] ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000451102100038
资助机构Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province
源URL[http://cas-ir.dicp.ac.cn/handle/321008/166506]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Li, Yuliang; Jiu, Tonggang
作者单位1.Shantou Univ, Key Lab Preparat & Applicat Ordered Struct Mat Gu, Shantou 515063, Guangdong, Peoples R China
2.Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
5.Shantou Univ, Dept Chem, Shantou 515063, Guangdong, Peoples R China
6.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Li, Yuliang,Li, Jiangsheng,Jiu, Tonggang,et al. Graphdiyne as a Host Active Material for Perovskite Solar Cell Application[J]. NANO LETTERS,2018,18(11):6941-6947.
APA Li, Yuliang.,Li, Jiangsheng.,Jiu, Tonggang.,Chen, Siqi.,Liu, Le.,...&Lu, Fushen.(2018).Graphdiyne as a Host Active Material for Perovskite Solar Cell Application.NANO LETTERS,18(11),6941-6947.
MLA Li, Yuliang,et al."Graphdiyne as a Host Active Material for Perovskite Solar Cell Application".NANO LETTERS 18.11(2018):6941-6947.

入库方式： OAI收割

来源：大连化学物理研究所

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