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Recent advances in direct catalytic hydrogenation of carbon dioxide to valuable C2+ hydrocarbons

文献类型：期刊论文

作者Guo, Lisheng1,2; Sun, Jian2; Ge, Qingjie2; Tsubaki, Noritatsu1
刊名JOURNAL OF MATERIALS CHEMISTRY A
出版日期2018-12-14
卷号6期号:46页码:23244-23262
ISSN号2050-7488
DOI10.1039/c8ta05377d
通讯作者Sun, Jian(sunj@dicp.ac.cn) ; Tsubaki, Noritatsu(tsubaki@eng.u-toyama.ac.jp)
英文摘要As one of the most effective methods, CO2 hydrogenation through heterogeneous catalysis is a promising means to mitigating the detrimental effects of anthropogenic CO2 that also accomplishes the effective recycling of carbon element. Considering the inertness of the CO2 molecule as well as the subsequent low chain propagation activity, the products are usually small molecules such as methane, methanol and formic acid. Furthermore, the imprecise regulation of C-C coupling further hinders the acquisition of target products. These problems make CO2 hydrogenation to useful C2+ hydrocarbons more challenging. Therefore, the rational design and fabrication of highly efficient and selective catalysts, including promoter-modified single metal catalysts, composite catalysts and bimetallic catalysts, is an inevitable process to upgrade the end products of CO2 utilization. This review will focus on the recent developments in the highly selective formation of C2+ hydrocarbons, especially the utilization of composite catalysts or multi-functional catalysts, which indicate the great potential derived from the synergistic effect of multi-active sites.
WOS关键词FISCHER-TROPSCH SYNTHESIS ; METHANOL SYNTHESIS CATALYST ; VALUE-ADDED PRODUCTS ; CO2 HYDROGENATION ; SELECTIVE CONVERSION ; LOWER OLEFINS ; COMPOSITE CATALYST ; IRON CATALYSTS ; LIGHT OLEFINS ; HETEROGENEOUS CATALYSTS
资助项目National Natural Science Foundation of China[21773234] ; National Natural Science Foundation of China[91745107] ; National Natural Science Foundation of China[21503215] ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA 21090203] ; Youth Innovation Promotion Association of Chinese Academy of Sciences[2018214] ; China Scholarship Council (CSC)[201704910797]
WOS研究方向Chemistry ; Energy & Fuels ; Materials Science
语种英语
WOS记录号WOS:000451813300005
出版者ROYAL SOC CHEMISTRY
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; China Scholarship Council (CSC) ; China Scholarship Council (CSC) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; China Scholarship Council (CSC) ; China Scholarship Council (CSC) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; China Scholarship Council (CSC) ; China Scholarship Council (CSC) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; China Scholarship Council (CSC) ; China Scholarship Council (CSC)
源URL[http://cas-ir.dicp.ac.cn/handle/321008/166588]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Sun, Jian; Tsubaki, Noritatsu
作者单位1.Univ Toyama, Sch Engn, Dept Appl Chem, Gofuku 3190, Toyama 9308555, Japan
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714		 Guo, Lisheng,Sun, Jian,Ge, Qingjie,et al. Recent advances in direct catalytic hydrogenation of carbon dioxide to valuable C2+ hydrocarbons[J]. JOURNAL OF MATERIALS CHEMISTRY A,2018,6(46):23244-23262.
APA Guo, Lisheng,Sun, Jian,Ge, Qingjie,&Tsubaki, Noritatsu.(2018).Recent advances in direct catalytic hydrogenation of carbon dioxide to valuable C2+ hydrocarbons.JOURNAL OF MATERIALS CHEMISTRY A,6(46),23244-23262.
MLA Guo, Lisheng,et al."Recent advances in direct catalytic hydrogenation of carbon dioxide to valuable C2+ hydrocarbons".JOURNAL OF MATERIALS CHEMISTRY A 6.46(2018):23244-23262.

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来源：大连化学物理研究所

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