中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 大连化学物理研究所
  3. 中国科学院大连化学物理研究所
Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules

文献类型：期刊论文

作者Ono, Luis K.1; Qi, Yabing1; Liu, Zonghao1; Qiu, Longbin1; Juarez-Perez, Emilio J.1; Hawash, Zafer1; Kim, Taehoon1; Jiang, Yan1; Wu, Zhifang1; Raga, Sonia R.1
刊名NATURE COMMUNICATIONS
出版日期2018-09-24
卷号9页码:11
ISSN号2041-1723
DOI10.1038/s41467-018-06317-8
通讯作者Qi, Yabing(Yabing.Qi@OIST.jp)
英文摘要Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 mu m in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 +/- 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cmx 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T-80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment.
WOS关键词ORGANOMETAL TRIHALIDE PEROVSKITE ; INORGANIC HALIDE PEROVSKITES ; METHYLAMINE-GAS ; SINGLE-CRYSTALS ; CH3NH3PBI3 ; STABILITY ; LIGHT ; INTERFACE ; TRANSPORT ; EVOLUTION
资助项目Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant[JP18K05266] ; 111 Project[B14041]
WOS研究方向Science & Technology - Other Topics
语种英语
WOS记录号WOS:000445329000015
出版者NATURE PUBLISHING GROUP
资助机构Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project
源URL[http://cas-ir.dicp.ac.cn/handle/321008/167010]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Qi, Yabing
作者单位1.Grad Univ, OIST, EMSSU, 1919-1 Tancha, Okinawa 9040495, Japan
2.Chinese Acad Sci, Dalian Inst Chem Phys, iChEM, Dalian Natl Lab Clean Energy, 457 Zhongshan Rd, Dalian 116023, Peoples R China
3.Shaanxi Normal Univ, Key Lab Appl Surface & Colloid Chem, Shaanxi Key Lab Adv Energy Devices,Sch Mat Sci &, Shaanxi Engn Lab Adv Energy Technol,Minist Educ, Xian 710119, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714		 Ono, Luis K.,Qi, Yabing,Liu, Zonghao,et al. Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules[J]. NATURE COMMUNICATIONS,2018,9:11.
APA Ono, Luis K..,Qi, Yabing.,Liu, Zonghao.,Qiu, Longbin.,Juarez-Perez, Emilio J..,...&Liu, Shengzhong .(2018).Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules.NATURE COMMUNICATIONS,9,11.
MLA Ono, Luis K.,et al."Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules".NATURE COMMUNICATIONS 9(2018):11.

入库方式： OAI收割

来源：大连化学物理研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。