Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid
文献类型：期刊论文
| 作者 | Wang, Wangyin1; Wang, Hong1,2; Zhu, Qingjun2,3; Qin, Wei1; Han, Guangye3; Shen, Jian-Ren3,4; Zong, Xu1; Li, Can1 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2016-08-01 |
| 卷号 | 55期号:32页码:9229-9233 |
| 关键词 | Photocatalysis Photoelectrochemistry Photosystem Ii Water Splitting Z-scheme |
| ISSN号 | 1433-7851 |
| DOI | 10.1002/anie.201604091 |
| 文献子类 | Article |
| 英文摘要 | Integrating natural and artificial photosynthetic platforms is an important approach to developing solar-driven hybrid systems with exceptional function over the individual components. A natural-artificial photosynthetic hybrid platform is formed by wiring photosystem II (PSII) and a platinum-decorated silicon photoelectrochemical (PEC) cell in a tandem manner based on a photocatalytic-PEC Z-scheme design. Although the individual components cannot achieve overall water splitting, the hybrid platform demonstrated the capability of unassisted solar-driven overall water splitting. Moreover, H-2 and O-2 evolution can be separated in this system, which is ascribed to the functionality afforded by the unconventional Z-scheme design. Furthermore, the tandem configuration and the spatial separation between PSII and artificial components provide more opportunities to develop efficient natural-artificial hybrid photosynthesis systems. |
| WOS关键词 | PHOTO-BIOELECTROCHEMICAL CELLS ; SHUTTLE REDOX MEDIATOR ; VISIBLE-LIGHT ; ELECTRON-TRANSFER ; Z-SCHEME ; OXYGEN ; SOLAR ; PHOTOCATALYSTS ; SYSTEM ; RESOLUTION |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000383371800017 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/168302]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Zong, Xu; Li, Can |
| 作者单位 | 1.Chinese Acad Sci, Collaborat Innovat Ctr Chem Energy Mat IChEM, Dalian Natl Lab Clean Energy, State Key Lab Catalysis,Dalian Inst Chem Phys, Zhongshan Rd 457, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Bot, Key Lab Photobiol, Photosynthesis Res Ctr, Beijing 100093, Peoples R China 4.Okayama Univ, Grad Sch Nat Sci & Technol, Photosynthesis Res Ctr, 1-1 Naka 3 Chome, Okayama 7008530, Japan |
| 推荐引用方式 GB/T 7714 | Wang, Wangyin,Wang, Hong,Zhu, Qingjun,et al. Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(32):9229-9233. |
| APA | Wang, Wangyin.,Wang, Hong.,Zhu, Qingjun.,Qin, Wei.,Han, Guangye.,...&Li, Can.(2016).Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(32),9229-9233. |
| MLA | Wang, Wangyin,et al."Spatially Separated Photosystem II and a Silicon Photoelectrochemical Cell for Overall Water Splitting: A Natural-Artificial Photosynthetic Hybrid".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.32(2016):9229-9233. |
入库方式： OAI收割
来源：大连化学物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。