Strategies for Efficient Charge Separation and Transfer in Artificial Photosynthesis of Solar Fuels
文献类型：期刊论文
| 作者 | Xu, Yuxing2,3; Li, Ailong2,3; Yao, Tingting2; Ma, Changtong2,3; Zhang, Xianwen2,3; Shah, Jafar Hussain2,3; Han, Hongxian1,2 |
| 刊名 | CHEMSUSCHEM
 |
| 出版日期 | 2017-11-23 |
| 卷号 | 10期号:22页码:4277-4305 |
| ISSN号 | 1864-5631 |
| 关键词 | Artificial Photosynthesis Charge Separation Co(2) Reduction Solar Fuels Water Splitting |
| DOI | 10.1002/cssc.201701598 |
| 文献子类 | Review |
| 英文摘要 | Converting sunlight to solar fuels by artificial photosynthesis is an innovative science and technology for renewable energy. Light harvesting, photogenerated charge separation and transfer (CST), and catalytic reactions are the three primary steps in the processes involved in the conversion of solar energy to chemical energy (SE-CE). Among the processes, CST is the key "energy pump and delivery" step in determining the overall solar-energy conversion efficiency. Efficient CST is always high priority in designing and assembling artificial photosynthesis systems for solar-fuel production. This Review not only introduces the fundamental strategies for CST but also the combinatory application of these strategies to five types of the most-investigated semiconductor-based artificial photosynthesis systems: particulate, Z-scheme, hybrid, photoelectrochemical, and photovoltaics-assisted systems. We show that artificial photosynthesis systems with high SE-CE efficiency can be rationally designed and constructed through combinatory application of these strategies, setting a promising blueprint for the future of solar fuels. |
| WOS关键词 | VISIBLE-LIGHT IRRADIATION ; PHOTOELECTROCHEMICAL WATER OXIDATION ; PHOTOCATALYTIC H-2 PRODUCTION ; SHUTTLE REDOX MEDIATOR ; DIFFERENT SEMICONDUCTOR PHOTOCATALYSTS ; ENERGY-CONVERSION EFFICIENCY ; DRIVEN HYDROGEN-PRODUCTION ; THIN-FILM ELECTRODES ; Z-SCHEME ; HIGHLY EFFICIENT |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000416158500004 |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/168340]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Han, Hongxian |
| 作者单位 | 1.Univ Chinese Acad Sci, Sch Future Technol, Beijing 100049, Peoples R China 2.Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xu, Yuxing,Li, Ailong,Yao, Tingting,et al. Strategies for Efficient Charge Separation and Transfer in Artificial Photosynthesis of Solar Fuels[J]. CHEMSUSCHEM,2017,10(22):4277-4305. |
| APA | Xu, Yuxing.,Li, Ailong.,Yao, Tingting.,Ma, Changtong.,Zhang, Xianwen.,...&Han, Hongxian.(2017).Strategies for Efficient Charge Separation and Transfer in Artificial Photosynthesis of Solar Fuels.CHEMSUSCHEM,10(22),4277-4305. |
| MLA | Xu, Yuxing,et al."Strategies for Efficient Charge Separation and Transfer in Artificial Photosynthesis of Solar Fuels".CHEMSUSCHEM 10.22(2017):4277-4305. |
入库方式： OAI收割
来源：大连化学物理研究所
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