Upgrading of derived pyrolysis vapors for the production of biofuels from corncobs
文献类型：期刊论文
| 作者 | Mao, Liaoyuan; Li, Yanxin; Zhang, Z. Conrad |
| 刊名 | FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING
 |
| 出版日期 | 2018-03-01 |
| 卷号 | 12期号:1页码:50-58 |
| 关键词 | Corncob Monolith Upgrading Pyrolysis |
| ISSN号 | 2095-0179 |
| DOI | 10.1007/s11705-017-1685-4 |
| 文献子类 | Article |
| 英文摘要 | A bubbling fluidized bed pyrolyzer was integrated with an in-situ honeycomb as a catalytic upgrading zone for the conversion of biomass to liquid fuels. In the upgrading zone, zeolite coated ceramic honeycomb (ZCCH) catalysts consisting of ZSM-5 (Si/Al = 25) were stacked and N-2 or recycled non-condensable gas was used as a carrier gas. Ground corncob particles were fast pyrolyzed in the bubbling bed using fine sand particles as a heat carrier and the resulting pyrolysis vapors were passed on-line over the catalytic upgrading zone. The influence of carrier gas, temperature, and weight hourly space velocity (WHSV) of catalyst on the oil product properties, distribution and mass balance were studied. Using ZCCH effectively increased the hydrocarbon yield and the heating value of the dry oil, especially in the presence of the recycled noncondensable gas. Even a low usage of zeolite catalyst at WSHV of 180 h(-1) was effective in upgrading the pyrolysis oil and other light olefins. The highest hydrocarbon (>= C2) and liquid aromatics yields reached to 14.23 and 4.17 wt-%, respectively. The undesirable products including light oxygenates, furans dramatically decreased in the presence of the ZCCH catalyst. |
| WOS关键词 | CATALYTIC FAST PYROLYSIS ; FLUIDIZED-BED REACTOR ; BIOMASS PYROLYSIS ; HZSM-5 ZEOLITE ; WOODY BIOMASS ; OIL ; TRANSFORMATION ; HYDROCARBONS ; HYDROGEN ; FUELS |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000425156500007 |
| 出版者 | SPRINGER |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/168664]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Zhang, Z. Conrad |
| 作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Mao, Liaoyuan,Li, Yanxin,Zhang, Z. Conrad. Upgrading of derived pyrolysis vapors for the production of biofuels from corncobs[J]. FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING,2018,12(1):50-58. |
| APA | Mao, Liaoyuan,Li, Yanxin,&Zhang, Z. Conrad.(2018).Upgrading of derived pyrolysis vapors for the production of biofuels from corncobs.FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING,12(1),50-58. |
| MLA | Mao, Liaoyuan,et al."Upgrading of derived pyrolysis vapors for the production of biofuels from corncobs".FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING 12.1(2018):50-58. |
入库方式： OAI收割
来源：大连化学物理研究所
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