Liquid-liquid two-phase flow in ultrasonic microreactors: Cavitation, emulsification, and mass transfer enhancement
文献类型:期刊论文
作者 | Zhao, Shuainan1,2; Dong, Zhengya1; Yao, Chaoqun1; Wen, Zhenghui1,2; Chen, Guangwen1; Yuan, Quan1 |
刊名 | AICHE JOURNAL |
出版日期 | 2018-04-01 |
卷号 | 64期号:4页码:1412-1423 |
ISSN号 | 0001-1541 |
关键词 | Ultrasound Cavitation Bubble Emulsification Hydrodynamic Behavior Mass Transfer Enhancement |
DOI | 10.1002/aic.16010 |
文献子类 | Article |
英文摘要 | The effects of ultrasound on the hydrodynamic and mass transfer behaviors of immiscible liquid-liquid two-phase flow was investigated in a domestic ultrasonic microreactor. Under ultrasonic irradiation, cavitation bubble was generated and underwent violent oscillation. Emulsification of immiscible phases was initiated by virtue of oscillating bubbles shuttling through the water/oil interface. The pressure drop was found to decrease with increasing ultrasound power, with a maximum decrement ratio of 12% obtained at power 30 W. The mass transfer behavior was characterized by extraction of Rhodamine B from water to 1-octanol. An enhancement factor of 1.3-2.2 on the overall mass-transfer coefficient was achieved under sonication. The mass transfer performance was comparable to passive microreactor at similar energy dissipation rate (61-184 W/kg). The extraction equilibrium was reached under a total flow velocity 0.01 m/s and input power 20 and 30 W, exhibiting its potential use in liquid-liquid extraction process. (c) 2017 American Institute of Chemical Engineers AIChE J, 64: 1412-1423, 2018 |
WOS关键词 | SUBMICRON MULTIPLE EMULSIONS ; PHASE-TRANSFER CATALYSIS ; GAS-LIQUID ; SLUG FLOW ; PRESSURE-DROP ; MICROSTRUCTURED REACTORS ; ACOUSTIC CAVITATION ; EXTRACTION ; INTENSIFICATION ; MICROCHANNELS |
WOS研究方向 | Engineering |
语种 | 英语 |
出版者 | WILEY |
WOS记录号 | WOS:000426489500022 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/168676] |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Chen, Guangwen |
作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
推荐引用方式 GB/T 7714 | Zhao, Shuainan,Dong, Zhengya,Yao, Chaoqun,et al. Liquid-liquid two-phase flow in ultrasonic microreactors: Cavitation, emulsification, and mass transfer enhancement[J]. AICHE JOURNAL,2018,64(4):1412-1423. |
APA | Zhao, Shuainan,Dong, Zhengya,Yao, Chaoqun,Wen, Zhenghui,Chen, Guangwen,&Yuan, Quan.(2018).Liquid-liquid two-phase flow in ultrasonic microreactors: Cavitation, emulsification, and mass transfer enhancement.AICHE JOURNAL,64(4),1412-1423. |
MLA | Zhao, Shuainan,et al."Liquid-liquid two-phase flow in ultrasonic microreactors: Cavitation, emulsification, and mass transfer enhancement".AICHE JOURNAL 64.4(2018):1412-1423. |
入库方式: OAI收割
来源:大连化学物理研究所
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