High-Rate Hydrogen Separation Using an MIEC Oxygen Permeable Membrane Reactor
文献类型：期刊论文
| 作者 | Cao, Zhongwei1; Yang, Weishen1; Li, Wenping1,2; Zhu, Xuefeng1 |
| 刊名 | AICHE JOURNAL
 |
| 出版日期 | 2017-04-01 |
| 卷号 | 63期号:4页码:1278-1286 |
| 关键词 | Hydrogen Separation Miec Membrane Reactor Water Splitting High-purity Hydrogen Oxygen Permeation |
| ISSN号 | 0001-1541 |
| DOI | 10.1002/aic.15502 |
| 文献子类 | Article |
| 英文摘要 | In this study, we propose using mixed ionic-electronic conducting (MIEC) oxygen permeable membrane to separate hydrogen via the water splitting reaction. To do that, steam was fed to one side of the membrane (side I) and a lowpurity hydrogen was fed to the other side (side II). Oxygen from water splitting on side I permeates through the membrane driven by an oxygen chemical potential gradient across the membrane to react with the low-purity hydrogen on side II. After condensation and drying, high-purity hydrogen is acquired from side I. Thus, the hydrogen separation process is realized based on the fact that the low-purity hydrogen is consumed and high-purity hydrogen is acquired. We achieved a high hydrogen separation rate (13.5 mL cm(-2) min(-1)) at 950 degrees C in a reactor equipped with a 0.5-mm-thick Ba0.98Ce0.05Fe0.95O3-delta membrane. This research proofed that it is feasible to upgrade hydrogen purity using an MIEC oxygen permeable membrane. (C) 2016 American Institute of Chemical Engineers AIChE J, 63: 1278-1286, 2017 |
| WOS关键词 | DUAL-PHASE MEMBRANES ; CONDUCTING MEMBRANES ; PALLADIUM MEMBRANES ; COMPOSITE MEMBRANES ; PARTIAL OXIDATION ; ENERGY ; PD ; PERMEATION ; STABILITY ; METHANE |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000398048500010 |
| 出版者 | WILEY |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/169284]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Yang, Weishen; Zhu, Xuefeng |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Cao, Zhongwei,Yang, Weishen,Li, Wenping,et al. High-Rate Hydrogen Separation Using an MIEC Oxygen Permeable Membrane Reactor[J]. AICHE JOURNAL,2017,63(4):1278-1286. |
| APA | Cao, Zhongwei,Yang, Weishen,Li, Wenping,&Zhu, Xuefeng.(2017).High-Rate Hydrogen Separation Using an MIEC Oxygen Permeable Membrane Reactor.AICHE JOURNAL,63(4),1278-1286. |
| MLA | Cao, Zhongwei,et al."High-Rate Hydrogen Separation Using an MIEC Oxygen Permeable Membrane Reactor".AICHE JOURNAL 63.4(2017):1278-1286. |
入库方式： OAI收割
来源：大连化学物理研究所
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