A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine
文献类型:期刊论文
作者 | Zhang, Ye5; Zhang, Wanshuo1,2; Gao, Shangyao2,3; Xie, Sujuan; Liu, Hui2,4; Zhu, Xiangxue2; Shang, Yongchen1; Liu, Shenglin2; Xu, Longya2 |
刊名 | CHINESE JOURNAL OF CATALYSIS
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出版日期 | 2017 |
卷号 | 38期号:1页码:168-175 |
关键词 | Binderless Zeolite Zsm-11 Amination Isobutene Tert-butylamine |
ISSN号 | 0253-9837 |
DOI | 10.1016/S1872-2067(17)62756-6 |
文献子类 | Article |
英文摘要 | A shaped binderless and two binder-containing ZSM-11 zeolite catalysts were prepared and characterized by powder X-ray diffraction,N-2 adsorption-desorption, and pyridine adsorption-infrared measurements. The binderless catalyst was synthesized using a dry-gel conversion technique, in which 1,6-hexanediamine and tetrabutylammonium bromide were used as structure-directing agents and no other alkaline materials were added. The catalytic performance of the zeolites in the direct amination of isobutene to tert-butylamine was evaluated in a fixed-bed reactor. By virtue of its high crystallinity as well as its good mechanical strength, the shaped binderless ZSM-11 catalyst showed a higher rate of formation of tert-butylamine than did the binder-containing catalysts. (C) 2017, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved. |
WOS关键词 | DIMETHYL ETHER ; METHANOL ; PERFORMANCE ; MORDENITE ; BENZENE ; SYSTEMS |
WOS研究方向 | Chemistry ; Engineering |
语种 | 英语 |
WOS记录号 | WOS:000394481400020 |
出版者 | SCIENCE PRESS |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/169508] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Shang, Yongchen; Liu, Shenglin |
作者单位 | 1.Harbin Normal Univ, Coll Chem & Chem Engn, Harbin 150025, Heilongjiang, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Sinochem Quanzhou Petrochem Co Ltd, Ctr Res & Dev, Quanzhou 362103, Fujian, Peoples R China 5.PetroChina Fushun Petrochem Co, Fushun 113008, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Ye,Zhang, Wanshuo,Gao, Shangyao,et al. A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine[J]. CHINESE JOURNAL OF CATALYSIS,2017,38(1):168-175. |
APA | Zhang, Ye.,Zhang, Wanshuo.,Gao, Shangyao.,Xie, Sujuan.,Liu, Hui.,...&Xu, Longya.(2017).A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine.CHINESE JOURNAL OF CATALYSIS,38(1),168-175. |
MLA | Zhang, Ye,et al."A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine".CHINESE JOURNAL OF CATALYSIS 38.1(2017):168-175. |
入库方式: OAI收割
来源:大连化学物理研究所
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