中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)

文献类型:期刊论文

作者Lu, Xingqiang3; Guo, Wei1,2; Wang, Xinlin1
刊名RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A
出版日期2017
卷号91期号:2页码:366-372
关键词Photoelectron Spectra State Populations Time-dependent Wave Packet Approach Three-level Ladder K-2 Molecule
ISSN号0036-0244
DOI10.1134/S0036024417020352
文献子类Article
英文摘要The delay time dependence of photoelectron spectra and state populations of three-level ladder K-2 molecule is investigated by pump-probe pulses via time-dependent wave packet approach. The periodical motion of the wave packet with oscillating period 500 fs results in the periodical variation of photoelectron spectra. The photoelectron spectra show Autler-Townes double splitting at zero delay time, and no splitting at positive delay time. The periodical change of state populations with delay time can be ascribed to the coupling effect between the two pulses. It is found that the selectivity of the state populations may be attained by regulating the delay time. The results can provide some important basis for realizing the optical control of molecules experimentally.
WOS关键词PROBE FEMTOSECOND SPECTROSCOPY ; ULTRASHORT LASER-PULSES ; WAVE-PACKET DYNAMICS ; ELECTRONIC STATES ; NA-2 MOLECULE ; EXCITED-STATES ; PHOTODISSOCIATION ; WAVEPACKET ; FIELDS ; NAK
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000395076500031
出版者MAIK NAUKA/INTERPERIODICA/SPRINGER
源URL[http://cas-ir.dicp.ac.cn/handle/321008/169564]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Lu, Xingqiang
作者单位1.Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China
2.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
3.Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China
推荐引用方式
GB/T 7714
Lu, Xingqiang,Guo, Wei,Wang, Xinlin. The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)[J]. RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A,2017,91(2):366-372.
APA Lu, Xingqiang,Guo, Wei,&Wang, Xinlin.(2017).The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1).RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A,91(2),366-372.
MLA Lu, Xingqiang,et al."The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)".RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A 91.2(2017):366-372.

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来源:大连化学物理研究所

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