Spatial distribution and quantum trajectory control of the molecular harmonic spectra
文献类型:期刊论文
作者 | Li, Wenliang1,4; Liu, Hang2; Castle, Rich-Samuel3; Feng, Liqiang1,2,3 |
刊名 | JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS
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出版日期 | 2016-12-01 |
卷号 | 25期号:4 |
关键词 | Molecular High-order Harmonic Spectra Spatial Distribution Quantum Trajectory Control Attosecond Pulse Spatial Inhomogeneous Effect |
ISSN号 | 0218-8635 |
DOI | 10.1142/S0218863516500533 |
文献子类 | Article |
英文摘要 | Spatial distribution and quantum trajectory control of the molecular harmonic spectra from H-2(+) are theoretically investigated through the combination of a few-cycle 800nm pulse and a half-cycle pulse. Results show that by properly adding the half-cycle pulse, the harmonic cutoffs from the recombination process are extended, and the harmonic intensities from the positive-x direction are suppressed. Moreover, as the internuclear distance increased, the modulations on the harmonic spectra are reduced. The time-dependent wave function and the time-frequency analyses of the harmonic spectra are shown to explain the above physical mechanism. Further, by adding the laser pulse to the bowtie-shaped gold nanostructure separated by an air gap g = 18nm, much higher harmonic cutoff order can be obtained in the positive-x(0) region. Finally, two isolated attosecond pulses with the full width at half maximum of 34 as and 31 as are obtained. |
WOS关键词 | ATTOSECOND PULSE GENERATION ; NONLINEAR OPTICS ; ASSISTED GENERATION ; LASER FIELDS ; ENHANCEMENT ; EMISSION ; UNIPOLAR |
WOS研究方向 | Optics ; Physics |
语种 | 英语 |
WOS记录号 | WOS:000394939300013 |
出版者 | WORLD SCIENTIFIC PUBL CO PTE LTD |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/169604] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Castle, Rich-Samuel |
作者单位 | 1.Chinese Acad Sci, State Key Lab Mol React Dynam, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 2.Liaoning Univ Technol, Sch Chem & Environm Engn, Jinzhou 121000, Peoples R China 3.Liaoning Univ Technol, Coll Sci, Jinzhou 121000, Peoples R China 4.Xinjiang Inst Engn, Key Lab, Univ Educ, Dept Xinjiang Uygur Autonomous Reg New Energy Mat, Urumqi 830091, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Wenliang,Liu, Hang,Castle, Rich-Samuel,et al. Spatial distribution and quantum trajectory control of the molecular harmonic spectra[J]. JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS,2016,25(4). |
APA | Li, Wenliang,Liu, Hang,Castle, Rich-Samuel,&Feng, Liqiang.(2016).Spatial distribution and quantum trajectory control of the molecular harmonic spectra.JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS,25(4). |
MLA | Li, Wenliang,et al."Spatial distribution and quantum trajectory control of the molecular harmonic spectra".JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS 25.4(2016). |
入库方式: OAI收割
来源:大连化学物理研究所
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