Highly efficient beta-SiC-supported 0.5% Rh-based catalyst for CO hydrogenation to C-2 oxygenates
文献类型：期刊论文
| 作者 | Chen, Weimiao1; Ding, Yunjie1,2; Xue, Fei1,3; Song, Xiangen1; Ning, Lili1 |
| 刊名 | CATALYSIS COMMUNICATIONS
 |
| 出版日期 | 2016-10-05 |
| 卷号 | 85页码:44-47 |
| 关键词 | Beta-sic Rh-based Catalyst Co Hydrogenation C-2 Oxygenates Low Rh Loading |
| ISSN号 | 1566-7367 |
| DOI | 10.1016/j.catcom.2016.07.016 |
| 文献子类 | Article |
| 英文摘要 | beta-SiC was used as a support for a 0.5% Rh-based catalyst for CO hydrogenation to C-2 oxygenates for the first time. The beta-SiC was acid etched and/or calcined at high temperature before use. The results show that the pretreatments had little effect on the textural and crystal properties of SiC, but calcination markedly increased the number of surface oxygen-containing groups. The pretreatment significantly increased the catalytic activities of SiC-supported Rh-Mn-Li/SiC catalysts in CO hydrogenation. An Rh efficiency of 97.2 g/g-Rh/h was achieved, the highest value reported in the literature to date. Possible reasons for this enhancement are suggested. (C) 2016 Elsevier B.V. All rights reserved. |
| WOS关键词 | FISCHER-TROPSCH SYNTHESIS ; ETHANOL-PRODUCTION ; SILICON-CARBIDE ; PERFORMANCE ; PROMOTION ; OXIDATION ; BEHAVIOR ; SURFACE ; SYNGAS ; NI |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000382594800011 |
| 出版者 | ELSEVIER SCIENCE BV |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/170070]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Ding, Yunjie |
| 作者单位 | 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Weimiao,Ding, Yunjie,Xue, Fei,et al. Highly efficient beta-SiC-supported 0.5% Rh-based catalyst for CO hydrogenation to C-2 oxygenates[J]. CATALYSIS COMMUNICATIONS,2016,85:44-47. |
| APA | Chen, Weimiao,Ding, Yunjie,Xue, Fei,Song, Xiangen,&Ning, Lili.(2016).Highly efficient beta-SiC-supported 0.5% Rh-based catalyst for CO hydrogenation to C-2 oxygenates.CATALYSIS COMMUNICATIONS,85,44-47. |
| MLA | Chen, Weimiao,et al."Highly efficient beta-SiC-supported 0.5% Rh-based catalyst for CO hydrogenation to C-2 oxygenates".CATALYSIS COMMUNICATIONS 85(2016):44-47. |
入库方式： OAI收割
来源：大连化学物理研究所
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