Ordered mesoporous alumina-supported bimetallic Pd-Ni catalysts for methane dry reforming reaction
文献类型：期刊论文
| 作者 | Ma, Qingxiang1,2; Sun, Jian3; Gao, Xinhua2; Zhang, Jianli1; Zhao, Tiansheng1; Yoneyama, Yoshiharu2; Tsubaki, Noritatsu2,4 |
| 刊名 | CATALYSIS SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2016 |
| 卷号 | 6期号:17页码:6542-6550 |
| ISSN号 | 2044-4753 |
| DOI | 10.1039/c6cy00841k |
| 文献子类 | Article |
| 英文摘要 | To compare the influence of Pd addition to Ni supported on ordered mesoporous alumina catalyst, prepared highly ordered mesoporous alumina (MA) was used as catalyst support for methane dry reforming under atmospheric pressure. Ni and Pd were impregnated on this support to obtain both monometallic and/or bimetallic catalysts, respectively. The fresh and spent catalysts were characterized by N-2 physical adsorption, high-resolution transmission electron microscopy(HRTEM), X-ray diffraction (XRD), H-2-temperature- programmed reduction (H-2-TPR), laser Raman spectroscopy and temperature-programmed hydrogenation (TPH). The XRD and HRTEM analysis results showed that Ni-Pd nanoalloy was formed after H-2 reduction. The catalytic performance analysis results indicated that the bimetallic nanoalloy catalysts showed higher activity than the monometallic catalyst. The deposition of carbon during the reaction was analyzed. The results indicated that different supported metal species led to different carbon species which influenced catalytic performance. |
| WOS关键词 | CARBON-DIOXIDE ; NI-CAO-ZRO2 CATALYST ; NICKEL-CATALYSTS ; CO2 ; HYDROGEN ; SYNGAS ; CH4 ; PERFORMANCE ; ALLOY |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000382025300011 |
| 出版者 | ROYAL SOC CHEMISTRY |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/170272]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Ma, Qingxiang; Tsubaki, Noritatsu |
| 作者单位 | 1.Ningxia Univ, State Key Lab Cultivat Base Nat Gas Convers, Yinchuan 750021, Peoples R China 2.Toyama Univ, Dept Appl Chem, Sch Engn, Gofuku 3190, Toyama 9308555, Japan 3.Chinese Acad Sci, Dalian Natl Lab Clean Energy DNL, Dalian Inst Chem Phys, Dalian 116023, Peoples R China 4.JST, ACT C, Tokyo 1028666, Japan |
| 推荐引用方式 GB/T 7714 | Ma, Qingxiang,Sun, Jian,Gao, Xinhua,et al. Ordered mesoporous alumina-supported bimetallic Pd-Ni catalysts for methane dry reforming reaction[J]. CATALYSIS SCIENCE & TECHNOLOGY,2016,6(17):6542-6550. |
| APA | Ma, Qingxiang.,Sun, Jian.,Gao, Xinhua.,Zhang, Jianli.,Zhao, Tiansheng.,...&Tsubaki, Noritatsu.(2016).Ordered mesoporous alumina-supported bimetallic Pd-Ni catalysts for methane dry reforming reaction.CATALYSIS SCIENCE & TECHNOLOGY,6(17),6542-6550. |
| MLA | Ma, Qingxiang,et al."Ordered mesoporous alumina-supported bimetallic Pd-Ni catalysts for methane dry reforming reaction".CATALYSIS SCIENCE & TECHNOLOGY 6.17(2016):6542-6550. |
入库方式： OAI收割
来源：大连化学物理研究所
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