Nitrogen-doped porous carbons with high performance for hydrogen storage
文献类型：期刊论文
| 作者 | Wang, Ziqiang1,2,3; Sun, Lixian2,3; Xu, Fen2; Zhou, Huaiying2; Peng, Xiaojun1; Sun, Dalin4; Wang, Jianchuan5; Du, Yong5 |
| 刊名 | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
 |
| 出版日期 | 2016-06-01 |
| 卷号 | 41期号:20页码:8489-8497 |
| 关键词 | Hydrochar Materials Koh Activation Porous Carbons Nitrogen-doped Hydrogen Storage |
| ISSN号 | 0360-3199 |
| DOI | 10.1016/j.ijhydene.2016.03.023 |
| 文献子类 | Article |
| 英文摘要 | Hydrothermally carbonized chitosan has been successfully used as a carbon source for the preparation of highly porous carbons via chemical activation. The porous carbons with different nitrogen contents (0.56-6.53 wt%) have high surface area (1362-3009 m(2) g(-1)) and large pore volume (0.670-1.497 cm(3) g(-1)). These properties can be varied from modifying the activation parameters (i.e., amount of activation agent and activation temperature). We observed hydrogen storage capacity of up to 2.71 wt% at 77 K and 1 bar, and 6.77 wt% at 20 bar, for PC-2-800 porous carbons. This result indicates that the hydrogen uptake of porous carbons mainly depends on the high micropore surface area related to optimum pore size. Furthermore, one found that high N-doping is beneficial for hydrogen storage at low pressure but it is detrimental at high pressure according to the analysis of hydrogen uptake isotherms. (C) 2016 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. |
| WOS关键词 | CARBIDE-DERIVED CARBON ; COVALENT ORGANIC FRAMEWORKS ; ACTIVATED CARBONS ; CHEMICAL ACTIVATION ; PORE-SIZE ; CAPACITY ; ADSORPTION ; NANOSTRUCTURES ; PRESSURE ; TEXTURE |
| WOS研究方向 | Chemistry ; Electrochemistry ; Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000377318800010 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/170614]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Sun, Lixian; Xu, Fen; Peng, Xiaojun |
| 作者单位 | 1.Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116024, Peoples R China 2.Guilin Univ Elect Technol, Guangxi Collaborat Innovat Ctr Struct & Property, Guangxi Key Lab Informat Mat, Sch Mat Sci & Engn, Guilin 541004, Peoples R China 3.Chinese Acad Sci, Dalian Inst Chem Phys, Mat & Thermochem Lab, 457 Zhongshan Rd, Dalian 116023, Peoples R China 4.Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China 5.Cent S Univ, Powder Met Res Inst, Changsha, Hunan, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Ziqiang,Sun, Lixian,Xu, Fen,et al. Nitrogen-doped porous carbons with high performance for hydrogen storage[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2016,41(20):8489-8497. |
| APA | Wang, Ziqiang.,Sun, Lixian.,Xu, Fen.,Zhou, Huaiying.,Peng, Xiaojun.,...&Du, Yong.(2016).Nitrogen-doped porous carbons with high performance for hydrogen storage.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,41(20),8489-8497. |
| MLA | Wang, Ziqiang,et al."Nitrogen-doped porous carbons with high performance for hydrogen storage".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 41.20(2016):8489-8497. |
入库方式： OAI收割
来源：大连化学物理研究所
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