Palladium on Nitrogen-Doped Mesoporous Carbon: A Bifunctional Catalyst for Formate-Based, Carbon-Neutral Hydrogen Storage
文献类型:期刊论文
作者 | Su, Xiong3; Wang, Fanan1,3; Xu, Jinming3; Shao, Xianzhao2,3; Huang, Yanqiang3; Zhang, Tao3 |
刊名 | CHEMSUSCHEM
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出版日期 | 2016-02-08 |
卷号 | 9期号:3页码:246-251 |
关键词 | Carbon Dioxide Fixation Doping Hydrogen Palladium Supported Catalysts |
ISSN号 | 1864-5631 |
DOI | 10.1002/cssc.201501376 |
文献子类 | Article |
英文摘要 | The lack of safe, efficient, and economical hydrogen storage technologies is a hindrance to the realization of the hydrogen economy. Reported herein is a reversible formate-based carbon-neutral hydrogen storage system that is established over a novel catalyst comprising palladium nanoparticles supported on nitrogen-doped mesoporous carbon. The support was fabricated by a hard template method and nitridated under a flow of ammonia. Detailed analyses demonstrate that this bicarbonate/formate redox equilibrium is promoted by the cooperative role of the doped nitrogen functionalities and the well-dispersed, electron-enriched palladium nanoparticles. |
WOS关键词 | FORMIC-ACID DECOMPOSITION ; OXYGEN REDUCTION REACTION ; ROOM-TEMPERATURE ; PD NANOPARTICLES ; EFFICIENT CATALYST ; AMBIENT CONDITIONS ; HIGH-PERFORMANCE ; AQUEOUS-SOLUTION ; FACILE SYNTHESIS ; GENERATION |
WOS研究方向 | Chemistry |
语种 | 英语 |
WOS记录号 | WOS:000370332400003 |
出版者 | WILEY-V C H VERLAG GMBH |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/171222] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Huang, Yanqiang; Zhang, Tao |
作者单位 | 1.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China 2.Shaanxi Univ Technol, Sch Chem & Environm Sci, Hanzhong 723001, Peoples R China 3.Chinese Acad Sci, State Key Lab Catalysis, Dalian Inst Chem Phys, 457 Zhongshan Rd, Dalian 116023, Peoples R China |
推荐引用方式 GB/T 7714 | Su, Xiong,Wang, Fanan,Xu, Jinming,et al. Palladium on Nitrogen-Doped Mesoporous Carbon: A Bifunctional Catalyst for Formate-Based, Carbon-Neutral Hydrogen Storage[J]. CHEMSUSCHEM,2016,9(3):246-251. |
APA | Su, Xiong,Wang, Fanan,Xu, Jinming,Shao, Xianzhao,Huang, Yanqiang,&Zhang, Tao.(2016).Palladium on Nitrogen-Doped Mesoporous Carbon: A Bifunctional Catalyst for Formate-Based, Carbon-Neutral Hydrogen Storage.CHEMSUSCHEM,9(3),246-251. |
MLA | Su, Xiong,et al."Palladium on Nitrogen-Doped Mesoporous Carbon: A Bifunctional Catalyst for Formate-Based, Carbon-Neutral Hydrogen Storage".CHEMSUSCHEM 9.3(2016):246-251. |
入库方式: OAI收割
来源:大连化学物理研究所
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