Fe-substituted Ba-hexaaluminates oxygen carrier for carbon dioxide capture by chemical looping combustion of methane
文献类型：期刊论文
| 作者 | Liu, Xin; Zhang, Tao; Tian, Ming; Wang, Xiaodong; Wang, Aiqin |
| 刊名 | AICHE JOURNAL
 |
| 出版日期 | 2016-03-01 |
| 卷号 | 62期号:3页码:792-801 |
| 关键词 | Chemical Looping Combustion Co2 Capture Iron Hexaaluminate Mirror Plane |
| ISSN号 | 0001-1541 |
| DOI | 10.1002/aic.15135 |
| 文献子类 | Article |
| 英文摘要 | Fe-substituted Ba-hexaaluninates (BFA-x (x=1-3), x indicates Fe content) oxygen carrier (OC) were found to exhibit excellent sintering-resistance under cyclic redox atmosphere at 800 degrees C thanks to the reservations of the structure during the CH4 reduction step, thus preventing the agglomeration of particles during the subsequent reoxidation step. Lattice oxygen highly active for the total combustion of CH4 was observed in the hexaaluminate structure and its chemical state was influenced by Fe content. The highest amount of active O coordinated with Fe3+ in the mirror plane (O-Fe3+(M)) for the total combustion was reacted (0.77 mmol/g) for BaFe3Al9O19 hexaaluminate OC. As a result, it exhibited the best reactivity with the CH4 conversion of 83% and CO2 selectivity of 100%. Moreover, superior regeneration and recyclability was also obtained, which originated from the fully recovery of O-Fe3+(M) in the hexaaluminate structure. (c) 2015 American Institute of Chemical Engineers AIChE J, 62: 792-801, 2016 |
| WOS关键词 | TEMPERATURE CATALYTIC COMBUSTION ; IN-SITU GASIFICATION ; FIXED-BED REACTOR ; CO2 CAPTURE ; IRON-OXIDE ; PARTIAL OXIDATION ; BARIUM HEXAALUMINATE ; SYNTHESIS GAS ; METAL-OXIDE ; MOSSBAUER-SPECTROSCOPY |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000370615300016 |
| 出版者 | WILEY-BLACKWELL |
| 源URL | [http://cas-ir.dicp.ac.cn/handle/321008/171228]  |
| 专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
| 通讯作者 | Wang, Xiaodong |
| 作者单位 | Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Xin,Zhang, Tao,Tian, Ming,et al. Fe-substituted Ba-hexaaluminates oxygen carrier for carbon dioxide capture by chemical looping combustion of methane[J]. AICHE JOURNAL,2016,62(3):792-801. |
| APA | Liu, Xin,Zhang, Tao,Tian, Ming,Wang, Xiaodong,&Wang, Aiqin.(2016).Fe-substituted Ba-hexaaluminates oxygen carrier for carbon dioxide capture by chemical looping combustion of methane.AICHE JOURNAL,62(3),792-801. |
| MLA | Liu, Xin,et al."Fe-substituted Ba-hexaaluminates oxygen carrier for carbon dioxide capture by chemical looping combustion of methane".AICHE JOURNAL 62.3(2016):792-801. |
入库方式： OAI收割
来源：大连化学物理研究所
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