中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
MoS2/sulfur and nitrogen co-doped reduced graphene oxide nanocomposite for enhanced electrocatalytic hydrogen evolution

文献类型:期刊论文

作者Ren, Xianpei2; Ren, Xiaodong2; Pang, Liuqing2; Zhang, Yunxia2; Ma, Qiang2; Fan, Haibo1,2; Liu, Shengzhong (Frank)2,3
刊名INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
出版日期2016-01-12
卷号41期号:2页码:916-923
关键词Molybdenum Disulfide Graphene Hydrogen Evolution Reaction Electrocatalyst
ISSN号0360-3199
DOI10.1016/j.ijhydene.2015.11.114
文献子类Article
英文摘要Cost-effective materials for electrocatalytic water splitting are key to renewable energy research. In this work, MoS2/sulfur and nitrogen co-doped reduced graphene oxide (SNG) nanocomposite was produced via a two-step hydrothermal process. The formation of nanocomposite was confirmed by X-ray diffraction (XRD), Raman spectroscopy, scanning electron microscopy (SEM), transmission electron microscopy (TEM). It is found that the MoS2/SNG nanocomposite exhibits much higher catalytic activity for the hydrogen evolution reaction (HER) relative to MoS2 and MoS2/RGO catalysts, as manifested by much larger cathodic current density with smaller overpotential of -120 mV and lower Tafel slope of 45 mV dec(-1). It is believed that the outstanding performance is attributed to the high electronic conductivity of SNG for fast charge transport. This study highlights the significance of the strong electronic coupling effect between the MoS2 and SNG in the enhancement of HER electrocatalytic activity. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
WOS关键词OXYGEN REDUCTION REACTIONS ; ACTIVE EDGE SITES ; MOS2 NANOPARTICLES ; MONOLAYER GRAPHENE ; WATER REDUCTION ; H-2 EVOLUTION ; FUEL-CELL ; MOLYBDENUM ; OXIDATION ; CATALYST
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
语种英语
WOS记录号WOS:000369202900019
出版者PERGAMON-ELSEVIER SCIENCE LTD
源URL[http://cas-ir.dicp.ac.cn/handle/321008/171414]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Liu, Shengzhong (Frank)
作者单位1.NW Univ Xian, Sch Phys, Xian 710069, Peoples R China
2.Shaanxi Normal Univ, Inst Adv Energy Mat, Key Lab Appl Surface & Colloid Chem, Natl Minist Educ,Sch Mat Sci & Engn, Xian 710119, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Ren, Xianpei,Ren, Xiaodong,Pang, Liuqing,et al. MoS2/sulfur and nitrogen co-doped reduced graphene oxide nanocomposite for enhanced electrocatalytic hydrogen evolution[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2016,41(2):916-923.
APA Ren, Xianpei.,Ren, Xiaodong.,Pang, Liuqing.,Zhang, Yunxia.,Ma, Qiang.,...&Liu, Shengzhong .(2016).MoS2/sulfur and nitrogen co-doped reduced graphene oxide nanocomposite for enhanced electrocatalytic hydrogen evolution.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,41(2),916-923.
MLA Ren, Xianpei,et al."MoS2/sulfur and nitrogen co-doped reduced graphene oxide nanocomposite for enhanced electrocatalytic hydrogen evolution".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 41.2(2016):916-923.

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来源:大连化学物理研究所

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