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Mild pyrolysis of ionic self-assembled cobalt porphyrins on carbon toward efficient electrochemical conversion of CO2 to CO

文献类型：期刊论文

作者Zhang, Xue3; Liu, Huiyuan1,2,3; Qin, Jiaqi3; Han, Hongsa3; Qiu, Chenxi3; Zhang, Siyu3; Hao, Xinyu3; Liu, Wei3; Song, Yujiang3
刊名CHEMICAL COMMUNICATIONS
出版日期2019-05-14
卷号55期号:39页码:5659-5662
ISSN号1359-7345
DOI10.1039/c9cc02156f
通讯作者Song, Yujiang(yjsong@dlut.edu.cn)
英文摘要We report ionic self-assembly of two oppositely charged cobalt(QIII) porphyrins (CoPs) on carbon coupled with subsequent mild pyrolysis at 350 degrees C, making CoPs lose some peripheral groups and become tightly adsorbed on the carbon with a high faradaic efficiency of 88 +/- 1.5% and a current density of 8 mA cm(-2) at a low overpotential of 430 mV toward electrochemical conversion of CO2 to CO.
WOS关键词COVALENT ORGANIC FRAMEWORKS ; N-C ; REDUCTION ; CATALYST ; DIOXIDE ; ELECTROREDUCTION ; PERFORMANCE ; NANOCRYSTALS ; NANOTUBES ; SITES
资助项目National Key Research & Development Program of China[2016YFB0101307] ; National Natural Science Foundation of China[21003114] ; National Natural Science Foundation of China[21103163] ; National Natural Science Foundation of China[21306188] ; National Natural Science Foundation of China[21373211] ; National Natural Science Foundation of China[21306187] ; Liaoning BaiQianWan Talents Program[201519] ; Program for Liaoning Excellent Talents in University[LR201514] ; Dalian Excellent Young Scientific and Technological Talents[2015R006] ; Fundamental Research Funds for the Central Universities[DUT15RC(3)001] ; Fundamental Research Funds for the Central Universities[DUT15ZD225]
WOS研究方向Chemistry
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000468401700026
资助机构National Key Research & Development Program of China ; National Key Research & Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; Program for Liaoning Excellent Talents in University ; Program for Liaoning Excellent Talents in University ; Dalian Excellent Young Scientific and Technological Talents ; Dalian Excellent Young Scientific and Technological Talents ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Key Research & Development Program of China ; National Key Research & Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; Program for Liaoning Excellent Talents in University ; Program for Liaoning Excellent Talents in University ; Dalian Excellent Young Scientific and Technological Talents ; Dalian Excellent Young Scientific and Technological Talents ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Key Research & Development Program of China ; National Key Research & Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; Program for Liaoning Excellent Talents in University ; Program for Liaoning Excellent Talents in University ; Dalian Excellent Young Scientific and Technological Talents ; Dalian Excellent Young Scientific and Technological Talents ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Key Research & Development Program of China ; National Key Research & Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Liaoning BaiQianWan Talents Program ; Liaoning BaiQianWan Talents Program ; Program for Liaoning Excellent Talents in University ; Program for Liaoning Excellent Talents in University ; Dalian Excellent Young Scientific and Technological Talents ; Dalian Excellent Young Scientific and Technological Talents ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities
源URL[http://cas-ir.dicp.ac.cn/handle/321008/171845]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Song, Yujiang
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Labs Clean Energy, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
3.Dalian Univ Technol, Sch Chem Engn, State Key Lab Fine Chem, 2 Linggong Rd, Dalian 116024, Peoples R China
推荐引用方式
GB/T 7714		 Zhang, Xue,Liu, Huiyuan,Qin, Jiaqi,et al. Mild pyrolysis of ionic self-assembled cobalt porphyrins on carbon toward efficient electrochemical conversion of CO2 to CO[J]. CHEMICAL COMMUNICATIONS,2019,55(39):5659-5662.
APA Zhang, Xue.,Liu, Huiyuan.,Qin, Jiaqi.,Han, Hongsa.,Qiu, Chenxi.,...&Song, Yujiang.(2019).Mild pyrolysis of ionic self-assembled cobalt porphyrins on carbon toward efficient electrochemical conversion of CO2 to CO.CHEMICAL COMMUNICATIONS,55(39),5659-5662.
MLA Zhang, Xue,et al."Mild pyrolysis of ionic self-assembled cobalt porphyrins on carbon toward efficient electrochemical conversion of CO2 to CO".CHEMICAL COMMUNICATIONS 55.39(2019):5659-5662.

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来源：大连化学物理研究所

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