中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Flexible thermal rectifier based on macroscopic PDMS@graphite composite film with asymmetric cone-shape interfaces

文献类型:期刊论文

作者Chen, Bensong1,2; Pawlik, Matthieu3; Tay, Roland Yingjie2; Zhu, Minmin4; Loeblein, Manuela4; Tsang, Siu Hon2; Teo, Edwin Hang Tong4,5
刊名CARBON
出版日期2018
卷号126期号:页码:464-471
ISSN号0008-6223
DOI10.1016/j.carbon.2017.10.046
英文摘要

Thermal rectifier is a device with the higher heat transport capacity in one direction than the backward one, being similar to the electrical diode working for the control of the electrical current. In this work, we report a new thermal rectifier based on the flexible macroscopic polydimethylsiloxane ( PDMS) film with asymmetric cone-shape holes embedded with micrometer sized graphite powder ( denoted as PDMS@graphite). The PDMS@graphite shows thermal rectification behavior with an extracted thermal rectification coefficient of 1.1326 +/- 0.009 under 129.8 K temperature bias, and this value can be further modulated by changing the asymmetric ratio of the cone-shape interface in the PDMS@graphite film. Two underlying mechanisms are invited to explain the thermal rectification effect in the PDMS@graphite system. The one is the opposite temperature dependence of thermal conductivity for PDMS and graphite powder. The other one is the different temperature dependent thermal conductivity of the asymmetric cone-shape graphite in PDMS@graphite film in the forward and backward heating direction when applying the same temperature bias, which can be demonstrated in the COMOSL theoretical simulated temperature distributions for the PDMS@graphite. The as-fabricated flexible macroscopic PDMS@graphite composite film thermal rectifier may provide the potential applications in thermal control and management. (C) 2017 Elsevier Ltd. All rights reserved.

WOS关键词RECTIFICATION ; NANOWIRES
资助项目NTU-A*STAR Silicon Technologies Centre of Excellence[1123510003] ; Singapore Ministry of Education Academic Research Fund[MOE2013-T2-2-050]
WOS研究方向Chemistry ; Materials Science
语种英语
WOS记录号WOS:000415319700053
出版者PERGAMON-ELSEVIER SCIENCE LTD
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/35813]  
专题合肥物质科学研究院_中科院固体物理研究所
通讯作者Teo, Edwin Hang Tong
作者单位1.Chinese Acad Sci, Inst Solid State Phys, Anhui Key Lab Nanomat & Nanotechnol, Key Lab Mat Phys,CAS Ctr Excellence Nanosci, Hefei 230031, Anhui, Peoples R China
2.Nanyang Technol Univ, Temasek Labs, 50 Nanyang Ave, Singapore 639798, Singapore
3.Nanyang Technol Univ, CNRS Int NTU Thales Res Alliance, 50 Nanyang Ave, Singapore 639798, Singapore
4.Nanyang Technol Univ, Sch Elect & Elect Engn, 50 Nanyang Ave, Singapore 639798, Singapore
5.Nanyang Technol Univ, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore
推荐引用方式
GB/T 7714
Chen, Bensong,Pawlik, Matthieu,Tay, Roland Yingjie,et al. Flexible thermal rectifier based on macroscopic PDMS@graphite composite film with asymmetric cone-shape interfaces[J]. CARBON,2018,126(无):464-471.
APA Chen, Bensong.,Pawlik, Matthieu.,Tay, Roland Yingjie.,Zhu, Minmin.,Loeblein, Manuela.,...&Teo, Edwin Hang Tong.(2018).Flexible thermal rectifier based on macroscopic PDMS@graphite composite film with asymmetric cone-shape interfaces.CARBON,126(无),464-471.
MLA Chen, Bensong,et al."Flexible thermal rectifier based on macroscopic PDMS@graphite composite film with asymmetric cone-shape interfaces".CARBON 126.无(2018):464-471.

入库方式: OAI收割

来源:合肥物质科学研究院

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