中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Lithium and its isotopes as tracers of groundwater salinization: A study in the southern coastal plain of Laizhou Bay, China

文献类型:期刊论文

作者Qi, Huihui1; Ma, Chuanming1; He, Zekang1,2,3; Hu, Xiaojing1; Gao, Lin1
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2019-02-10
卷号650页码:878-890
关键词Southern coastal plain of Laizhou Bay Groundwater salinization Hydrochemistry Lithium isotope Brine and seawater intrusion
ISSN号0048-9697
DOI10.1016/j.scitotenv.2018.09.122
通讯作者Ma, Chuanming(machuanming@cug.edu.cn)
英文摘要In the southern coastal plain of Laizhou Bay, due to intensive exploitation of groundwater since the early 1970s, the shallow aquifer has been severely influenced by saltwater intrusion, which causes the extraction to shift from shallow to deeper aquifer changing the hydrogeological condition greatly. This study was conducted to investigate the groundwater salinization using hydrochemistry and H, O and Li isotope data. Dissolved Li shows a linear correlation with Cl and Br in seawater, brine and saline groundwater indicating the marine Li source, whereas the enrichment of Li in surface water, brackish and fresh groundwater is impacted by dissolution of silicate minerals. The analyses of hydrochemistry and isotopes (H, O and Li) indicate that brine originated from seawater evaporation, followed by mixing processes and some water-rock interactions; shallow saline groundwater originated from brine diluted with seawater and fresh groundwater; deep saline groundwater originated from seawater intrusion. The negative correlation of delta(7) Li and Li/Na in surface water, brackish and fresh groundwater is contrary to the general conclusion, indicating the slow weathering of silicate minerals and hydraulic interaction between surface water and shallow groundwater in this area. The analyses of hydrochemistry and isotopes (Li, H and O) can well identify the salinity sources and isotope fractionation in groundwater flow and mixing, especially groundwater with high TDS. As both mixing with saltwater and isotope fractionation can explain the combination of high delta(7) Li and low TDS in brackish groundwater, isotope fractionation may limit their use in recognizing salinity sources of groundwater with low TDS. (C) 2018 Elsevier B.V. All rights reserved.
WOS关键词CANADIAN SHIELD BRINES ; WEATHERING PROCESSES ; SEAWATER CHEMISTRY ; WATER-INTRUSION ; STABLE-ISOTOPES ; VOLCANIC-ROCKS ; BORON ISOTOPES ; ORGANIC-ACIDS ; MURRAY BASIN ; LI ISOTOPES
资助项目National Natural Science Foundation of China[41572212]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000447092700091
出版者ELSEVIER SCIENCE BV
资助机构National Natural Science Foundation of China
源URL[http://ir.igsnrr.ac.cn/handle/311030/52815]  
专题中国科学院地理科学与资源研究所
通讯作者Ma, Chuanming
作者单位1.China Univ Geosci, Sch Environm Studies, Wuhan 430074, Hubei, Peoples R China
2.Chinese Acad Sci, Key Lab Water Cycle & Related Land Surface Proc, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China
3.Univ Chinese Acad Sci, Coll Resources & Environm, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Qi, Huihui,Ma, Chuanming,He, Zekang,et al. Lithium and its isotopes as tracers of groundwater salinization: A study in the southern coastal plain of Laizhou Bay, China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,650:878-890.
APA Qi, Huihui,Ma, Chuanming,He, Zekang,Hu, Xiaojing,&Gao, Lin.(2019).Lithium and its isotopes as tracers of groundwater salinization: A study in the southern coastal plain of Laizhou Bay, China.SCIENCE OF THE TOTAL ENVIRONMENT,650,878-890.
MLA Qi, Huihui,et al."Lithium and its isotopes as tracers of groundwater salinization: A study in the southern coastal plain of Laizhou Bay, China".SCIENCE OF THE TOTAL ENVIRONMENT 650(2019):878-890.

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来源:地理科学与资源研究所

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