中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Behavior of N-ethyl perfluorooctane sulfonamido acetic acid (N-EtFOSAA) in biosolids amended soil-plant microcosms of seven plant species: Accumulation and degradation

文献类型:期刊论文

作者Pan, Ying; Shi, Xiaoli; Wen, Bei; Zhan, Hongna; Hu, Xiaoyu; Huang, Honglin; Lv, Jitao; Zhang, Shuzhen
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2018-11-15
卷号642页码:366-373
ISSN号0048-9697
关键词N-EtFOSAA Soil Plant Accumulation Degradation
文献子类Article
英文摘要Perfluorooctane sulfonate (PFOS) precursors have been found extensively in sewage sludge and biosolids-amended soils. The degradation of these precursors are regarded as a significant source of PFOS in the environment. In this study, the accumulation of N-ethyl perfluorooctane sulfonamido acetic acid (N-EtFOSAA) in the plants of seven species, namely alfalfa, lettuce, maize, mung bean, radish, ryegrass, and soybean from biosolids-amended soil, and the degradation kinetics of N-EtFOSAA in soil-plant microcosms were evaluated over 60 days. N-EtFOSAA was found in the roots of all plant species, while was not in stems and leaves. The root concentration factors of N-EtFOSAA ranged 0.52-1.37 (pmol/g(root))(pmol/g(root)). Stepwise multiple regression analysis was used to elucidate the accumulation of N-EtFOSAA in the roots of plants. The results showed that the root protein and lipid contents explain 85.0% of the variation in root N-EtFOSAA levels (P < 0.05). Four degradation products, including N-ethyl perfluorooctane sulfonamide (N-EtFOSA), perfluorooctane sulfonamide acetate (FOSAA), perfluorooctane sulfonamide (FOSA) and PFOS were found in soils and plant roots, stems and leaves, indicating the degradation of N-EtFOSAA in soil-plant system. Degradation kinetics fitted a first-order kinetic model well. Degradation rate constants of N-EtFOSAA in the microcosms with plants ranged 0.063-0.165 d(-1), which was 1.40-3.6 times higher than those without plants. Degradation rate constant of maize was relatively higher than those of other plant species. The results is the first to reveal N-EtFOSAA accumulation in plants and degradation in soil-plant microcosms. (C) 2018 Elsevier B.V. All rights reserved.
源URL[http://ir.rcees.ac.cn/handle/311016/40885]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
推荐引用方式
GB/T 7714
Pan, Ying,Shi, Xiaoli,Wen, Bei,et al. Behavior of N-ethyl perfluorooctane sulfonamido acetic acid (N-EtFOSAA) in biosolids amended soil-plant microcosms of seven plant species: Accumulation and degradation[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2018,642:366-373.
APA Pan, Ying.,Shi, Xiaoli.,Wen, Bei.,Zhan, Hongna.,Hu, Xiaoyu.,...&Zhang, Shuzhen.(2018).Behavior of N-ethyl perfluorooctane sulfonamido acetic acid (N-EtFOSAA) in biosolids amended soil-plant microcosms of seven plant species: Accumulation and degradation.SCIENCE OF THE TOTAL ENVIRONMENT,642,366-373.
MLA Pan, Ying,et al."Behavior of N-ethyl perfluorooctane sulfonamido acetic acid (N-EtFOSAA) in biosolids amended soil-plant microcosms of seven plant species: Accumulation and degradation".SCIENCE OF THE TOTAL ENVIRONMENT 642(2018):366-373.

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来源:生态环境研究中心

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