Synthesis of biomass tar-derived foams through spontaneous foaming for ultra-efficient herbicide removal from aqueous solution
文献类型：期刊论文
| 作者 | Li, Dong1,2; Li, Yi3; Liu, Hongjun4,5; Ma, Jing1,2; Liu, Zhengang1,2; Gai, Chao1,2; Jiao, Wentao1,2 |
| 刊名 | SCIENCE OF THE TOTAL ENVIRONMENT
 |
| 出版日期 | 2019-07-10 |
| 卷号 | 673页码:110-119 |
| 关键词 | Waste biomass tar Carbon foam Adsorption Organic herbicide |
| ISSN号 | 0048-9697 |
| DOI | 10.1016/j.scitotenv.2019.04.057 |
| 英文摘要 | Pyrolysis is one of the most important approaches to convert waste biomass into renewable energy and biomaterials, and the tar is the inevitable by-product of this process. In this study, carbon foams were prepared innovatively with biomass tar as the precursor through spontaneous gas foaming approach and used for dicamba removal from aqueous solution. The results showed that prepared carbon foams had unique properties including rich microporous structure and high specific surface area (reaching 1667 m(2)/g). In addition, the prepared carbons had high thermal stability due to the high graphitic degree. The adsorption results indicated that pH showed a great effect on the adsorption of dicamba onto the prepared carbon foams. The carbon foam exhibited ultra-fast dicamba removal and ultra-high adsorption capacity of 891.74 mg/g at room temperature. The adsorption process was well described by pseudo-second-order kinetics and Langmuir isotherm models. The thermodynamic study indicated dicamba adsorption onto the prepared carbon foams was a spontaneous and exothermic process. In addition, the good reusability from recovery test demonstrated that the prepared carbon foams had promising potential for dicamba removal from aqueous solution. (C) 2019 Elsevier B.V. All rights reserved. |
| WOS关键词 | ACTIVATED CARBON ; ZINC HYDROXIDE ; POROUS CARBONS ; FAST PYROLYSIS ; ADSORPTION ; PITCH ; CELLULOSE ; KOH ; REDUCTION ; CHROMIUM |
| 资助项目 | "100 Talents" Program of the Chinese Academy of Sciences[Y5N41I1C01] |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000466418300013 |
| 出版者 | ELSEVIER SCIENCE BV |
| 资助机构 | "100 Talents" Program of the Chinese Academy of Sciences |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/28143]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Liu, Zhengang; Jiao, Wentao |
| 作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, 18 Shuangqing Rd, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 4.Henan Univ, Key Lab Natl Med & Immunoengn Henan Prov, Kaifeng 475004, Henan, Peoples R China 5.AGplus Technol Co Ptd, Water Technol Res Ctr, 303 Longhai Er Rd, Huizhou 516082, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Dong,Li, Yi,Liu, Hongjun,et al. Synthesis of biomass tar-derived foams through spontaneous foaming for ultra-efficient herbicide removal from aqueous solution[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2019,673:110-119. |
| APA | Li, Dong.,Li, Yi.,Liu, Hongjun.,Ma, Jing.,Liu, Zhengang.,...&Jiao, Wentao.(2019).Synthesis of biomass tar-derived foams through spontaneous foaming for ultra-efficient herbicide removal from aqueous solution.SCIENCE OF THE TOTAL ENVIRONMENT,673,110-119. |
| MLA | Li, Dong,et al."Synthesis of biomass tar-derived foams through spontaneous foaming for ultra-efficient herbicide removal from aqueous solution".SCIENCE OF THE TOTAL ENVIRONMENT 673(2019):110-119. |
入库方式： OAI收割
来源：过程工程研究所
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