中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 过程工程研究所
  3. 中国科学院过程工程研究所
Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics

文献类型：期刊论文

作者Wang, Jian1; Zhao, Hainan1,3; Liu, Xiaolong1; Xu, Wenqing1,2; Guo, Yangyang1; Song, Jianfei3; Zhu, Tingyu1,2
刊名CATALYSIS LETTERS
出版日期2019-07-01
卷号149期号:7页码:2004-2014
关键词Ruthenium Ru TiO2 Catalytic oxidation Benzene Chlorobenzene
ISSN号1011-372X
DOI10.1007/s10562-019-02802-x
英文摘要In this work, we presented a detailed evaluation of Ru/TiO2 (P25) catalysts for the catalytic oxidation of (chloro)-aromatics. The model catalysts were synthesized through wet impregnation. Catalytic evaluations, as well as ICP, BET, XRD and TEM analyses, were conducted. The results indicated that RuO2 tended to be distributed on the rutile phase of TiO2, leading to an inhomogeneous distribution. These Ru/TiO2 catalysts were very active, especially for chlorobenzene oxidation. The conversions of benzene and chlorobenzene were both suppressed by the introduction of additional water. But the amount of polychlorinated benzenes as by-products was also reduced. However, the activity of the catalyst significantly decreased with an increase in calcination temperature, suggesting that the thermal stability of the catalyst still needed to be improved. [GRAPHICS] .
WOS关键词RUTHENIUM CATALYSTS ; RU/CEO2 CATALYSTS ; AMMONIA-SYNTHESIS ; LOW-TEMPERATURE ; COMBUSTION ; CHLOROBENZENE ; VOCS ; CO ; EMISSION ; KINETICS
资助项目National Natural Science Foundation of China[51708540] ; Key Research Program of the Chinese Academy of Sciences[ZDRW-ZS-2017-6-2]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000468172400026
出版者SPRINGER
资助机构National Natural Science Foundation of China ; Key Research Program of the Chinese Academy of Sciences
源URL[http://ir.ipe.ac.cn/handle/122111/28149]  
专题中国科学院过程工程研究所
通讯作者Wang, Jian; Zhu, Tingyu
作者单位1.Chinese Acad Sci, Beijing Res Ctr Proc Pollut Control, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing 100190, Peoples R China
2.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
3.China Univ Petr, Coll Mech & Transportat Engn, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China
推荐引用方式
GB/T 7714		 Wang, Jian,Zhao, Hainan,Liu, Xiaolong,et al. Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics[J]. CATALYSIS LETTERS,2019,149(7):2004-2014.
APA Wang, Jian.,Zhao, Hainan.,Liu, Xiaolong.,Xu, Wenqing.,Guo, Yangyang.,...&Zhu, Tingyu.(2019).Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics.CATALYSIS LETTERS,149(7),2004-2014.
MLA Wang, Jian,et al."Study on the Catalytic Properties of Ru/TiO2 Catalysts for the Catalytic Oxidation of (Chloro)-Aromatics".CATALYSIS LETTERS 149.7(2019):2004-2014.

入库方式： OAI收割

来源：过程工程研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。