中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Numerical simulation of reactive mixing process in a stirred reactor with the DQMOM-IEM model

文献类型:期刊论文

作者Duan, Xiaoxia1,2; Feng, Xin1,2; Mao, Zai-Sha1; Yang, Chao1,2
刊名CHEMICAL ENGINEERING JOURNAL
出版日期2019-03-15
卷号360页码:1177-1187
关键词Mixing DQMOM-IEM Stirred reactor Mathematical modeling Computational fluid dynamics Micro-mixing
ISSN号1385-8947
DOI10.1016/j.cej.2018.10.156
英文摘要The direct quadrature method of moments combined with the interaction by exchange with the mean model (named as DQMOM-IEM) is applied to simulate the novel reactive-PLIF (planar laser induced fluorescence) experiment in an unbaffled stirred reactor. By using the mixture fraction and reaction progress variables, the descriptions of the Fenton reaction and oxidation reaction of Rhodamine B are formulated. The quenching of fluorescent signal can be visualized by solving the probability, probability weighted mixture fraction and reaction progress variables used in the two-environment DQMOM coupled with the IEM micro-mixing model. The effect of impeller speed on the mixing and reactions are revealed by the simulated dynamic processes. The predictions by DQMOM-IEM micro-mixing model agree well with the experimental data, suggesting that this model is an effective approach for numerical prediction of turbulent reactive flow in stirred reactors.
WOS关键词LASER-INDUCED FLUORESCENCE ; PARALLEL CHEMICAL-REACTIONS ; LIQUID-PHASE ; TURBULENT-FLOW ; POWER-CONSUMPTION ; EDDY SIMULATION ; TANK ; CFD ; TIME ; VESSELS
资助项目National Key Research and Development Program[2016YFB0301702] ; National Natural Science Foundation of China[21776282] ; National Natural Science Foundation of China[21490584] ; National Natural Science Foundation of China[21808221] ; Major National Scientific Instrument Development Project[21427814] ; Key Research Program of Frontier Sciences, CAS[QYZDJ-SSW-JSC030] ; Jiangsu National Synergetic Innovation Center for Advanced Materials ; Open Project Program of Beijing Key Laboratory of Enze Biomass Fine Chemicals
WOS研究方向Engineering
语种英语
WOS记录号WOS:000460964000117
出版者ELSEVIER SCIENCE SA
资助机构National Key Research and Development Program ; National Natural Science Foundation of China ; Major National Scientific Instrument Development Project ; Key Research Program of Frontier Sciences, CAS ; Jiangsu National Synergetic Innovation Center for Advanced Materials ; Open Project Program of Beijing Key Laboratory of Enze Biomass Fine Chemicals
源URL[http://ir.ipe.ac.cn/handle/122111/28287]  
专题中国科学院过程工程研究所
通讯作者Feng, Xin
作者单位1.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Duan, Xiaoxia,Feng, Xin,Mao, Zai-Sha,et al. Numerical simulation of reactive mixing process in a stirred reactor with the DQMOM-IEM model[J]. CHEMICAL ENGINEERING JOURNAL,2019,360:1177-1187.
APA Duan, Xiaoxia,Feng, Xin,Mao, Zai-Sha,&Yang, Chao.(2019).Numerical simulation of reactive mixing process in a stirred reactor with the DQMOM-IEM model.CHEMICAL ENGINEERING JOURNAL,360,1177-1187.
MLA Duan, Xiaoxia,et al."Numerical simulation of reactive mixing process in a stirred reactor with the DQMOM-IEM model".CHEMICAL ENGINEERING JOURNAL 360(2019):1177-1187.

入库方式: OAI收割

来源:过程工程研究所

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