中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings

文献类型:期刊论文

作者Chen, Zhong1,2; Zhou, Jianqiang2; Chen, Zeliang2; Chen, Hongzhen2; Chen, Qiao2; He, Chunlan4; Liu, Xiaoling3; Yuanjian, Xu1,2
刊名Journal of Environmental Chemical Engineering
出版日期2018
卷号6期号:5页码:6691-6699
DOI10.1016/j.jece.2018.10.040
英文摘要Oil-based drill cuttings (OBDC), which originate from drilling operations in oil and gas fields, have been included in the 2016 National Hazardous Waste Inventory of China. In this investigation, the decontamination of two typical OBDC samples from shale gas fields, i.e., a diesel type from a vertical well (A) and a white oil type from a horizontal well (B), was conducted using superheated steam at near-saturation pressure. The effects of different pressures (0.6-5.5 MPa), temperatures (175-225 °C), and water flow rates (2-8 ml min-1) on the removal efficiency were studied in a semi-continuous laboratory apparatus. The results indicated that temperature was the most important parameter, followed by water flow rate and pressure. The OBDC characteristics also significantly affected the removal efficiency. Both the superheated steam and subcritical water present during treatment removed not only all extractable organics but also some other organics. With the optimal parameters of 2.3 MPa, 225 °C, and 6 ml min-1, 78.56% and 83.09% of total organic carbon were removed from A and B, respectively. After treatment, the OBDCs were not hazardous any more as their oil content has dropped to almost zero. Further analysis confirmed that this method possessed the advantages of solvent extraction (excellent solubility) and thermal desorption (high temperature). The results of X-ray diffraction and Sanning electron microscopy indicated that the microstructure and crystalline structure of in-organics in OBDC were not obviously changed during the treatment. As a result, this method can be considered as a new potential separation technique for treatment of OBDC. © 2018 Published by Elsevier Ltd.
电子版国际标准刊号22133437
语种英语
源URL[http://119.78.100.138/handle/2HOD01W0/8026]  
专题环境友好化学过程研究中心
作者单位1.State Key Laboratory of Petroleum Pollution Control, Beijing; 102206, China;
2.Key Laboratory of Reservoir Aquatic Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing; 400714, China;
3.Chongqing Academy of Chinese Materia Medica, NO. 34Huangjueya, Nan' An District, Chongqing; 400065, China;
4.Chongqing Institute for Food and Drug Control, Chongqing; 401120, China
推荐引用方式
GB/T 7714
Chen, Zhong,Zhou, Jianqiang,Chen, Zeliang,et al. A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings[J]. Journal of Environmental Chemical Engineering,2018,6(5):6691-6699.
APA Chen, Zhong.,Zhou, Jianqiang.,Chen, Zeliang.,Chen, Hongzhen.,Chen, Qiao.,...&Yuanjian, Xu.(2018).A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings.Journal of Environmental Chemical Engineering,6(5),6691-6699.
MLA Chen, Zhong,et al."A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings".Journal of Environmental Chemical Engineering 6.5(2018):6691-6699.

入库方式: OAI收割

来源:重庆绿色智能技术研究院

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