A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings
文献类型:期刊论文
作者 | Chen, Zhong1,2; Zhou, Jianqiang2; Chen, Zeliang2; Chen, Hongzhen2; Chen, Qiao2; He, Chunlan4; Liu, Xiaoling3; Yuanjian, Xu1,2 |
刊名 | Journal of Environmental Chemical Engineering |
出版日期 | 2018 |
卷号 | 6期号:5页码:6691-6699 |
DOI | 10.1016/j.jece.2018.10.040 |
英文摘要 | Oil-based drill cuttings (OBDC), which originate from drilling operations in oil and gas fields, have been included in the 2016 National Hazardous Waste Inventory of China. In this investigation, the decontamination of two typical OBDC samples from shale gas fields, i.e., a diesel type from a vertical well (A) and a white oil type from a horizontal well (B), was conducted using superheated steam at near-saturation pressure. The effects of different pressures (0.6-5.5 MPa), temperatures (175-225 °C), and water flow rates (2-8 ml min-1) on the removal efficiency were studied in a semi-continuous laboratory apparatus. The results indicated that temperature was the most important parameter, followed by water flow rate and pressure. The OBDC characteristics also significantly affected the removal efficiency. Both the superheated steam and subcritical water present during treatment removed not only all extractable organics but also some other organics. With the optimal parameters of 2.3 MPa, 225 °C, and 6 ml min-1, 78.56% and 83.09% of total organic carbon were removed from A and B, respectively. After treatment, the OBDCs were not hazardous any more as their oil content has dropped to almost zero. Further analysis confirmed that this method possessed the advantages of solvent extraction (excellent solubility) and thermal desorption (high temperature). The results of X-ray diffraction and Sanning electron microscopy indicated that the microstructure and crystalline structure of in-organics in OBDC were not obviously changed during the treatment. As a result, this method can be considered as a new potential separation technique for treatment of OBDC. © 2018 Published by Elsevier Ltd. |
电子版国际标准刊号 | 22133437 |
语种 | 英语 |
源URL | [http://119.78.100.138/handle/2HOD01W0/8026] |
专题 | 环境友好化学过程研究中心 |
作者单位 | 1.State Key Laboratory of Petroleum Pollution Control, Beijing; 102206, China; 2.Key Laboratory of Reservoir Aquatic Environment, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing; 400714, China; 3.Chongqing Academy of Chinese Materia Medica, NO. 34Huangjueya, Nan' An District, Chongqing; 400065, China; 4.Chongqing Institute for Food and Drug Control, Chongqing; 401120, China |
推荐引用方式 GB/T 7714 | Chen, Zhong,Zhou, Jianqiang,Chen, Zeliang,et al. A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings[J]. Journal of Environmental Chemical Engineering,2018,6(5):6691-6699. |
APA | Chen, Zhong.,Zhou, Jianqiang.,Chen, Zeliang.,Chen, Hongzhen.,Chen, Qiao.,...&Yuanjian, Xu.(2018).A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings.Journal of Environmental Chemical Engineering,6(5),6691-6699. |
MLA | Chen, Zhong,et al."A laboratory evaluation of superheated steam extraction process for decontamination of oil-based drill cuttings".Journal of Environmental Chemical Engineering 6.5(2018):6691-6699. |
入库方式: OAI收割
来源:重庆绿色智能技术研究院
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