Facile and Green Synthesis of Palladium Nanoparticles-Graphene-Carbon Nanotube Material with High Catalytic Activity
文献类型：期刊论文
| 作者 | Sun, Tai1; Zhang, Zheye1; Xiao, Junwu1; Chen, Chen1; Xiao, Fei1; Wang, Shuai1,2; Liu, Yunqi3 |
| 刊名 | SCIENTIFIC REPORTS
 |
| 出版日期 | 2013-08-28 |
| 卷号 | 3 |
| ISSN号 | 2045-2322 |
| DOI | 10.1038/srep02527 |
| 英文摘要 | We report a facile and green method to synthesize a new type of catalyst by coating Pd nanoparticles (NPs) on reduced graphene oxide (rGO)-carbon nanotube (CNT) nanocomposite. An rGO-CNT nanocomposite with three-dimensional microstructures was obtained by hydrothermal treatment of an aqueous dispersion of graphene oxide (GO) and CNTs. After the rGO-CNT composites have been dipped in K2PdCl4 solution, the spontaneous redox reaction between the GO-CNT and PdCl42- led to the formation of nanohybrid materials consisting rGO-CNT decorated with 4 nm Pd NPs, which exhibited excellent and stable catalytic activity: the reduction of 4-nitrophenol to 4-aminophenol using NaBH4 as a catalyst was completed in only 20 s at room temperature, even when the Pd content of the catalyst was 1.12 wt%. This method does not require rigorous conditions or toxic agents and thus is a rapid, efficient, and green approach to the fabrication of highly active catalysts. |
| 语种 | 英语 |
| WOS记录号 | WOS:000323596800007 |
| 出版者 | NATURE PUBLISHING GROUP |
| 源URL | [http://ir.iccas.ac.cn/handle/121111/42062]  |
| 专题 | 中国科学院化学研究所 |
| 通讯作者 | Wang, Shuai |
| 作者单位 | 1.Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China 2.Huazhong Univ Sci & Technol, Sch Mech Sci & Engn, State Key Lab Digital Mfg Equipment & Technol, Wuhan 430074, Peoples R China 3.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Tai,Zhang, Zheye,Xiao, Junwu,et al. Facile and Green Synthesis of Palladium Nanoparticles-Graphene-Carbon Nanotube Material with High Catalytic Activity[J]. SCIENTIFIC REPORTS,2013,3. |
| APA | Sun, Tai.,Zhang, Zheye.,Xiao, Junwu.,Chen, Chen.,Xiao, Fei.,...&Liu, Yunqi.(2013).Facile and Green Synthesis of Palladium Nanoparticles-Graphene-Carbon Nanotube Material with High Catalytic Activity.SCIENTIFIC REPORTS,3. |
| MLA | Sun, Tai,et al."Facile and Green Synthesis of Palladium Nanoparticles-Graphene-Carbon Nanotube Material with High Catalytic Activity".SCIENTIFIC REPORTS 3(2013). |
入库方式： OAI收割
来源：化学研究所
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